一种催化自由基介导的N-氧化反应的双核锰簇合物。 - Suppr

A binuclear manganese cluster that catalyzes radical-mediated N-oxygenation.

作者信息

Winkler Robert, Zocher Georg, Richter Ingrid, Friedrich Thorsten, Schulz Georg E, Hertweck Christian

机构信息

Department of Biomolecular Chemistry, Leibniz Institute for Natural Product Research and Infection Biology (HKI), Beutenbergstrasse 11a, 07745 Jena, Germany.

出版信息

Angew Chem Int Ed Engl. 2007;46(45):8605-8. doi: 10.1002/anie.200703089.

DOI:10.1002/anie.200703089

PMID:17926312

Abstract

摘要

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A binuclear manganese cluster that catalyzes radical-mediated N-oxygenation.

作者信息

Winkler Robert, Zocher Georg, Richter Ingrid, Friedrich Thorsten, Schulz Georg E, Hertweck Christian

机构信息

Department of Biomolecular Chemistry, Leibniz Institute for Natural Product Research and Infection Biology (HKI), Beutenbergstrasse 11a, 07745 Jena, Germany.

出版信息

Angew Chem Int Ed Engl. 2007;46(45):8605-8. doi: 10.1002/anie.200703089.

DOI:10.1002/anie.200703089

PMID:17926312

Abstract

摘要

相似文献

A binuclear manganese cluster that catalyzes radical-mediated N-oxygenation.

Angew Chem Int Ed Engl. 2007;46(45):8605-8. doi: 10.1002/anie.200703089.

Structure and action of the N-oxygenase AurF from Streptomyces thioluteus.

J Mol Biol. 2007 Oct 12;373(1):65-74. doi: 10.1016/j.jmb.2007.06.014. Epub 2007 Jun 9.

Highly stereoselective epoxidation with H2O2 catalyzed by electron-rich aminopyridine manganese catalysts.

Org Lett. 2013 Dec 20;15(24):6158-61. doi: 10.1021/ol403018x. Epub 2013 Nov 18.

AurF from Streptomyces thioluteus and a possible new family of manganese/iron oxygenases.

Biochemistry. 2007 Sep 18;46(37):10413-8. doi: 10.1021/bi701060g. Epub 2007 Aug 24.

A diiron center stabilized by a bis-TPA ligand as a model of soluble methane monooxygenase: predominant alkene epoxidation with H2O2.

Angew Chem Int Ed Engl. 2005 Nov 4;44(43):7104-6. doi: 10.1002/anie.200501825.

Manganese(III)-catalyzed free radical reactions on trimetallic nitride endohedral metallofullerenes.

J Am Chem Soc. 2007 Dec 19;129(50):15710-7. doi: 10.1021/ja0768439. Epub 2007 Nov 21.

Effect of additives on chemoselectivity and diastereoselectivity in the catalytic epoxidation of chiral allylic alcohols with hydrogen peroxide and binuclear manganese complexes.

J Org Chem. 2009 Feb 6;74(3):1135-40. doi: 10.1021/jo801974e.

DNA binding and catalytic properties of positively charged corroles.

Angew Chem Int Ed Engl. 2007;46(23):4320-4. doi: 10.1002/anie.200700757.

Manganese and iron flavonolates as flavonol 2,4-dioxygenase mimics.

Chem Commun (Camb). 2007 Dec 28(48):5235-7. doi: 10.1039/b711864c. Epub 2007 Oct 11.

Manganese(III)-mediated direct phosphonation of arylalkenes and arylalkynes.

Chem Commun (Camb). 2010 Mar 14;46(10):1721-3. doi: 10.1039/b925951a. Epub 2010 Feb 8.

引用本文的文献

Direct aromatic nitration by bacterial P450 enzymes.

Methods Enzymol. 2023;693:307-337. doi: 10.1016/bs.mie.2023.09.008. Epub 2023 Oct 12.

Diiron monooxygenases in natural product biosynthesis.

Nat Prod Rep. 2018 Jul 18;35(7):646-659. doi: 10.1039/C7NP00061H.

Heteroatom-Heteroatom Bond Formation in Natural Product Biosynthesis.

Chem Rev. 2017 Apr 26;117(8):5784-5863. doi: 10.1021/acs.chemrev.6b00621. Epub 2017 Apr 4.

Crystal structure of CmlI, the arylamine oxygenase from the chloramphenicol biosynthetic pathway.

J Biol Inorg Chem. 2016 Sep;21(5-6):589-603. doi: 10.1007/s00775-016-1363-x. Epub 2016 May 26.

Mechanism for Six-Electron Aryl-N-Oxygenation by the Non-Heme Diiron Enzyme CmlI.

J Am Chem Soc. 2016 Jun 15;138(23):7411-21. doi: 10.1021/jacs.6b03341. Epub 2016 Jun 3.

Four-electron oxidation of p-hydroxylaminobenzoate to p-nitrobenzoate by a peroxodiferric complex in AurF from Streptomyces thioluteus.

Proc Natl Acad Sci U S A. 2010 Sep 7;107(36):15722-7. doi: 10.1073/pnas.1002785107. Epub 2010 Aug 23.

Metalloenzymes: Natural product nitrosation.

Nat Chem Biol. 2010 Sep;6(9):636-7. doi: 10.1038/nchembio.425.

A long-lived, substrate-hydroxylating peroxodiiron(III/III) intermediate in the amine oxygenase, AurF, from Streptomyces thioluteus.

J Am Chem Soc. 2009 Sep 30;131(38):13608-9. doi: 10.1021/ja9064969.

In vitro reconstitution and crystal structure of p-aminobenzoate N-oxygenase (AurF) involved in aureothin biosynthesis.

Proc Natl Acad Sci U S A. 2008 May 13;105(19):6858-63. doi: 10.1073/pnas.0712073105. Epub 2008 May 5.

A binuclear manganese cluster that catalyzes radical-mediated N-oxygenation.

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A binuclear manganese cluster that catalyzes radical-mediated N-oxygenation.

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