Inosov D S, Fink J, Kordyuk A A, Borisenko S V, Zabolotnyy V B, Schuster R, Knupfer M, Büchner B, Follath R, Dürr H A, Eberhardt W, Hinkov V, Keimer B, Berger H
Institute for Solid State Research, IFW Dresden, P.O. Box 270116, D-01171 Dresden, Germany.
Phys Rev Lett. 2007 Dec 7;99(23):237002. doi: 10.1103/PhysRevLett.99.237002. Epub 2007 Dec 6.
Using high-resolution angle-resolved photoemission spectroscopy we have studied the momentum and photon energy dependence of the anomalous high-energy dispersion, termed waterfalls, between the Fermi level and 1 eV binding energy in several high-T_{c} superconductors. We observe strong changes of the dispersion between different Brillouin zones and a strong dependence on the photon energy around 75 eV, which we associate with the resonant photoemission at the Cu3p-->3d_{x;{2}-y;{2}} edge. We conclude that the high-energy "waterfall" dispersion results from a strong suppression of the photoemission intensity at the center of the Brillouin zone due to matrix element effects and is, therefore, not an intrinsic feature of the spectral function. This indicates that the new high-energy scale in the electronic structure of cuprates derived from the waterfall-like dispersion may be incorrect.
利用高分辨率角分辨光电子能谱,我们研究了几种高温超导体中费米能级与1电子伏特结合能之间反常高能色散(称为瀑布)的动量和光子能量依赖性。我们观察到不同布里渊区之间色散的强烈变化以及对75电子伏特左右光子能量的强烈依赖性,我们将其与Cu3p→3dx²-y²边缘处的共振光电子发射联系起来。我们得出结论,高能“瀑布”色散是由于矩阵元效应导致布里渊区中心光电子发射强度强烈抑制的结果,因此不是光谱函数的固有特征。这表明从类似瀑布的色散推导出来的铜酸盐电子结构中的新高能标度可能是不正确的。