Hellén H, Hakola H, Haaparanta S, Pietarila H, Kauhaniemi M
Finnish Meteorological Institute, Air Quality, Helsinki, Finland.
Sci Total Environ. 2008 Apr 15;393(2-3):283-90. doi: 10.1016/j.scitotenv.2008.01.019. Epub 2008 Feb 12.
The importance of wood combustion to local air quality was estimated by measuring different air pollutants and conducting chemical mass balance modelling. PM10, PM2.5, PAHs and VOC concentrations in ambient air were measured in a typical Finnish residential area. Measurements were conducted in January-March 2006. For some compounds, wood combustion was clearly the main local source at this site. The effect of wood combustion was more clearly seen for organic compounds than for fine particle mass. For fine particles, background concentrations dominated. However, very high, short-lived concentration peaks were detected, when the wind direction and other weather conditions were favourable. For organic compounds, the effect of wood combustion was seen in diurnal and in two-week average concentrations. PAH-concentrations were often several times higher at the residential area than in the background. Benzene concentrations showed similar diurnal pattern as the use of wood and benzene/toluene ratios indicated that wood combustion is the most important source. A chemical mass balance model was used for studying the effect of wood combustion on the measured concentrations of VOCs. Model results showed that the main local sources for VOCs at Kurkimäki are wood combustion and traffic. Wood combustion was clearly the most important source for many compounds (e.g., benzene).
通过测量不同的空气污染物并进行化学质量平衡建模,估算了木材燃烧对当地空气质量的影响。在芬兰一个典型的居民区测量了环境空气中的PM10、PM2.5、多环芳烃(PAHs)和挥发性有机化合物(VOCs)浓度。测量于2006年1月至3月进行。对于某些化合物,木材燃烧显然是该地点主要的本地污染源。木材燃烧对有机化合物的影响比对细颗粒物质量的影响更为明显。对于细颗粒物,背景浓度占主导。然而,当风向和其他天气条件有利时,会检测到非常高的、短暂的浓度峰值。对于有机化合物,木材燃烧的影响在日浓度和两周平均浓度中都能看到。居民区的多环芳烃浓度通常比背景浓度高出几倍。苯浓度呈现出与木材使用相似的日变化模式,苯/甲苯比值表明木材燃烧是最重要的来源。使用化学质量平衡模型研究木材燃烧对所测挥发性有机化合物浓度的影响。模型结果表明,库尔基马基挥发性有机化合物的主要本地来源是木材燃烧和交通。木材燃烧显然是许多化合物(如苯)最重要的来源。