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具有圆角的银纳米棱镜的光强度增强特性。

Characteristics of light intensity enhancement of a silver nanoprism with rounded corners.

作者信息

Yamaguchi K, Inoue T, Fujii M, Ogawa T, Matsuzaki Y, Okamoto T, Haraguchi M, Fukui M

机构信息

Department of Optical Science and Technology, Faculty of Engineering, The University of Tokushima, 2-1 Minami-josanjima, Tokushima 770-8506, Japan.

出版信息

J Microsc. 2008 Mar;229(Pt 3):545-50. doi: 10.1111/j.1365-2818.2008.01941.x.

Abstract

We have fabricated silver nanoprisms of 100-600 nm side length by focussed ion beam lithography and measured the light intensity scattering spectra using dark-field microscopy. Two resonance peaks due to localized surface plasmon excitation were observed in the spectra and their central frequency shown to depend on the prism size. The near-field electromagnetic intensity distribution with TE-polarized light at the vacuum wavelength of 632.8 nm was measured. We have obtained a much lower light intensity enhancement than previously numerically predicated. However, scattering spectra obtained numerically, taking into account roundness of the prism corners, agree well with experimental ones. At the same time, the numerically determined field distribution was different to the near-field intensity obtained experimentally. Our results suggest the particular shape of the corner region of the prism is a key factor for obtaining a large light intensity enhancement and shaping the local field distribution.

摘要

我们通过聚焦离子束光刻技术制备了边长为100 - 600纳米的银纳米棱镜,并使用暗场显微镜测量了光强散射光谱。在光谱中观察到了由于局域表面等离子体激元激发产生的两个共振峰,并且它们的中心频率显示出依赖于棱镜尺寸。测量了在真空波长632.8纳米下TE偏振光的近场电磁强度分布。我们获得的光强增强比之前数值预测的要低得多。然而,考虑到棱镜角部的圆度通过数值计算得到的散射光谱与实验光谱吻合得很好。同时,数值确定的场分布与实验获得的近场强度不同。我们的结果表明,棱镜角部区域的特定形状是获得大光强增强和塑造局部场分布的关键因素。

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