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交通和气象对近道路空气质量的影响:罗利近道路研究的方法与趋势总结

Traffic and meteorological impacts on near-road air quality: summary of methods and trends from the Raleigh Near-Road Study.

作者信息

Baldauf Richard, Thoma Eben, Hays Michael, Shores Richard, Kinsey John, Gullett Brian, Kimbrough Sue, Isakov Vlad, Long Thomas, Snow Richard, Khlystov Andrey, Weinstein Jason, Chen Fu-Lin, Seila Robert, Olson David, Gilmour Ian, Cho Seung-Hyun, Watkins Nealson, Rowley Patricia, Bang John

机构信息

U.S. Environmental Protection Agency, Office of Research and Development, National Risk Management Research Laboratory, Research Triangle Park, NC 27711, USA.

出版信息

J Air Waste Manag Assoc. 2008 Jul;58(7):865-78. doi: 10.3155/1047-3289.58.7.865.

Abstract

A growing number of epidemiological studies conducted worldwide suggest an increase in the occurrence of adverse health effects in populations living, working, or going to school near major roadways. A study was designed to assess traffic emissions impacts on air quality and particle toxicity near a heavily traveled highway. In an attempt to describe the complex mixture of pollutants and atmospheric transport mechanisms affecting pollutant dispersion in this near-highway environment, several real-time and time-integrated sampling devices measured air quality concentrations at multiple distances and heights from the road. Pollutants analyzed included U.S. Environmental Protection Agency (EPA)-regulated gases, particulate matter (coarse, fine, and ultrafine), and air toxics. Pollutant measurements were synchronized with real-time traffic and meteorological monitoring devices to provide continuous and integrated assessments of the variation of near-road air pollutant concentrations and particle toxicity with changing traffic and environmental conditions, as well as distance from the road. Measurement results demonstrated the temporal and spatial impact of traffic emissions on near-road air quality. The distribution of mobile source emitted gas and particulate pollutants under all wind and traffic conditions indicated a higher proportion of elevated concentrations near the road, suggesting elevated exposures for populations spending significant amounts of time in this microenvironment. Diurnal variations in pollutant concentrations also demonstrated the impact of traffic activity and meteorology on near-road air quality. Time-resolved measurements of multiple pollutants demonstrated that traffic emissions produced a complex mixture of criteria and air toxic pollutants in this microenvironment. These results provide a foundation for future assessments of these data to identify the relationship of traffic activity and meteorology on air quality concentrations and population exposures.

摘要

全球范围内越来越多的流行病学研究表明,在主要道路附近居住、工作或上学的人群中,不良健康影响的发生率有所增加。一项研究旨在评估交通排放对一条繁忙高速公路附近空气质量和颗粒物毒性的影响。为了描述影响该高速公路附近环境中污染物扩散的复杂污染物混合物和大气传输机制,几个实时和时间积分采样装置在距离道路不同距离和高度处测量了空气质量浓度。分析的污染物包括美国环境保护局(EPA)监管的气体、颗粒物(粗颗粒物、细颗粒物和超细颗粒物)以及空气有毒物质。污染物测量与实时交通和气象监测装置同步,以提供对近道路空气污染物浓度和颗粒物毒性随交通和环境条件变化以及与道路距离变化的连续和综合评估。测量结果证明了交通排放在时间和空间上对近道路空气质量的影响。在所有风和交通条件下,移动源排放的气体和颗粒物污染物分布表明,道路附近高浓度污染物的比例更高,这表明在这个微环境中长时间停留的人群暴露水平较高。污染物浓度的日变化也证明了交通活动和气象对近道路空气质量的影响。对多种污染物的时间分辨测量表明,交通排放在这个微环境中产生了由标准污染物和空气有毒污染物组成的复杂混合物。这些结果为未来评估这些数据以确定交通活动和气象与空气质量浓度及人群暴露之间的关系奠定了基础。

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