Liu Xiuhong, Peng Yi, Wu Changyong, Akio Takigawa, Peng Yongzhen
School of Municipal and Environmental Engineering, Harbin Institute of Technology, Harbin 150090, China.
J Environ Sci (China). 2008;20(6):641-5. doi: 10.1016/s1001-0742(08)62106-3.
The production of N2O during nitrogen removal from real domestic wastewater was investigated in a lab-scale aerobic-anoxic sequencing batch reactor with a working volume of 14 L. The results showed that the total N2O-N production reached higher than 1.87 mg/L, and up to 4% of removed nitrogen was converted into N2O. In addition, N2O led to a much higher greenhouse effect than CO2 during aerobic reaction phase, this proved that N2O production could not be neglected. The N2O-N production during nitrification was 1.85 mg/L, whereas, during denitrification, no N2O was produced, nitrification was the main source of N2O production during nitrogen removal. Furthermore, during denitrification, the dissolved N2O at the end of aeration was found to be further reduced to N2. Denitrification thus had the potential of controlling N2O production.
在一个工作体积为14升的实验室规模的好氧-缺氧序批式反应器中,研究了实际生活污水脱氮过程中N2O的产生情况。结果表明,N2O-N的总产生量达到了1.87毫克/升以上,高达4%的去除氮被转化为N2O。此外,在好氧反应阶段,N2O导致的温室效应比CO2高得多,这证明N2O的产生不容忽视。硝化过程中N2O-N的产生量为1.85毫克/升,而在反硝化过程中,未产生N2O,硝化是脱氮过程中N2O产生的主要来源。此外,在反硝化过程中,曝气结束时溶解的N2O被发现进一步还原为N2。因此,反硝化具有控制N2O产生的潜力。