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正交钙钛矿锰氧化物a轴极化铁电相中的摆线自旋序

Cycloidal spin order in the a-axis polarized ferroelectric phase of orthorhombic perovskite manganite.

作者信息

Yamasaki Y, Sagayama H, Abe N, Arima T, Sasai K, Matsuura M, Hirota K, Okuyama D, Noda Y, Tokura Y

机构信息

Department of Applied Physics, University of Tokyo, Tokyo 113-8656, Japan.

出版信息

Phys Rev Lett. 2008 Aug 29;101(9):097204. doi: 10.1103/PhysRevLett.101.097204.

DOI:10.1103/PhysRevLett.101.097204
PMID:18851653
Abstract

The ferroelectric state in an orthorhombic perovskite RMnO3 (R=Gd0.7Tb0.3) was proved by neutron scattering studies to show the cycloidal spin state with the ab-spiral plane and the spin-helicity dependent polarization vector along the a axis, sharing the microscopic origin (inverse Dzyaloshinskii-Moriya interaction) with the more widely observed P||c state (e.g., for R=Tb and Dy) with the bc-spiral plane. The magnetic-field induced polarization flop from P||c to P||a as well known for RMnO3 is thus assigned to the orthogonal flop of the spin spiral plane from bc to ab.

摘要

中子散射研究证明,正交钙钛矿RMnO₃(R = Gd₀.₇Tb₀.₃)中的铁电态显示出具有ab螺旋平面的摆线自旋态,以及沿a轴的自旋螺旋度相关极化矢量,它与更广泛观察到的具有bc螺旋平面的P||c态(例如,对于R = Tb和Dy)具有相同的微观起源(反Dzyaloshinskii-Moriya相互作用)。因此,RMnO₃中众所周知的磁场诱导极化从P||c翻转到P||a,被归因于自旋螺旋平面从bc到ab的正交翻转。

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