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东马来西亚海洋沉积物中天然存在的放射性核素活度浓度分布。

Distribution of naturally occurring radionuclides activity concentration in East Malaysian marine sediment.

作者信息

Yii M W, Zaharudin A, Abdul-Kadir I

机构信息

Malaysian Nuclear Agency (Nuclear Malaysia), Bangi, 43000 Kajang, Malaysia.

出版信息

Appl Radiat Isot. 2009 Apr;67(4):630-5. doi: 10.1016/j.apradiso.2008.11.019. Epub 2008 Dec 24.

Abstract

Studies of naturally occurring radioactive materials (NORM) distribution of (226)Ra, (228)Ra and (40)K in East Malaysia were carried out as part of a marine coastal environment project. The results of measurements will serve as baseline data and background reference level for Malaysia coastlines. Sediments from 21 coastal locations and 10 near shore locations were collected for analyses. The samples were dried, finely ground, sealed in a container and stored for a minimum of 30 days to establish secular equilibrium between (226)Ra and (228)Ra and their respective radioactive progenies. They were counted using a high-purity germanium (HPGe) spectrometer covering the respective progeny energy peak. For (40)K, the presence of this was measured directly via its 1460 keV energy peak. The concentration of (226)Ra, (228)Ra and (40)K in samples obtained from coastal Sarawak ranged between 23 and 41 (mean 30+/-2) Bq/kg, 27 and 45 (mean 39+/-4) Bq/kg and 142 and 680 (mean 462+/-59) Bq/kg, respectively. Meanwhile, the concentration of (226)Ra, (228)Ra and (40)K for samples obtained from coastal Sabah ranged between 16 and 30 (mean 23+/-2) Bq/kg, 23 and 45 (mean 35+/-4) Bq/kg and 402 and 842 (mean 577+/-75) Bq/kg, respectively. For the Sarawak near shore stations, the concentration of (226)Ra, (228)Ra and (40)K ranged between 11 and 36 (mean 22+/-2) Bq/kg, 21 and 65 (mean 39+/-5) Bq/kg and 149 and 517 (mean 309+/-41) Bq/kg, respectively. Meanwhile, the concentration of (226)Ra, (228)Ra and (40)K for samples obtained from Sabah ranged between 9 and 31 (mean 14+/-2) Bq/kg, 10 and 48 (mean 21+/-3) Bq/kg and 140 and 580 (mean 269+/-36) Bq/kg, respectively. The calculated external hazard values of between 0.17 and 0.33 (less than unity) showed that there is little risk of external hazard to the workers handling the sediments.

摘要

作为海洋海岸环境项目的一部分,对东马来西亚天然存在的放射性物质(NORM)中镭-226、镭-228和钾-40的分布进行了研究。测量结果将作为马来西亚海岸线的基线数据和背景参考水平。采集了21个沿海地点和10个近岸地点的沉积物进行分析。样品经干燥、研磨成细粉后,密封于容器中,并至少保存30天,以建立镭-226和镭-228与其各自放射性子体之间的长期平衡。使用覆盖各自子体能量峰的高纯锗(HPGe)光谱仪对样品进行计数。对于钾-40,直接通过其1460keV能量峰测量其存在情况。从砂拉越沿海采集的样品中,镭-226、镭-228和钾-40的浓度分别在23至41(平均30±2)Bq/kg、27至45(平均39±4)Bq/kg和142至680(平均462±59)Bq/kg之间。同时,从沙巴沿海采集的样品中,镭-226、镭-228和钾-40的浓度分别在16至30(平均23±2)Bq/kg、23至45(平均35±4)Bq/kg和402至842(平均577±75)Bq/kg之间。对于砂拉越近岸站点,镭-226、镭-228和钾-40的浓度分别在11至36(平均22±2)Bq/kg、21至65(平均39±5)Bq/kg和149至517(平均309±41)Bq/kg之间。同时,从沙巴采集的样品中,镭-226、镭-228和钾-40的浓度分别在9至31(平均14±2)Bq/kg、10至48(平均21±3)Bq/kg和140至580(平均269±36)Bq/kg之间。计算得出的外部危害值在0.17至0.33之间(小于1),表明处理沉积物的工人面临的外部危害风险很小。

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