Hoppler J, Stahn J, Niedermayer Ch, Malik V K, Bouyanfif H, Drew A J, Rössle M, Buzdin A, Cristiani G, Habermeier H-U, Keimer B, Bernhard C
Physics Department and Fribourg Center for Nanomaterials (FriMat), Fribourg University, Chemin du Musée 3, CH-1700 Fribourg, Switzerland.
Nat Mater. 2009 Apr;8(4):315-9. doi: 10.1038/nmat2383. Epub 2009 Feb 15.
Artificial multilayers offer unique opportunities for combining materials with antagonistic orders such as superconductivity and ferromagnetism and thus to realize novel quantum states. In particular, oxide multilayers enable the utilization of the high superconducting transition temperature of the cuprates and the versatile magnetic properties of the colossal-magnetoresistance manganites. However, apart from exploratory work, the in-depth investigation of their unusual properties has only just begun. Here we present neutron reflectometry measurements of a Y(0.6)Pr(0.4)Ba(2)Cu(3)O(7) (10 nm)/La(2/3)Ca(1/3)MnO(3) (10 nm) superlattice, which reveal a surprisingly large superconductivity-induced modulation of the vertical ferromagnetic magnetization profile. Most surprisingly, this modulation seems to involve the density rather than the orientation of the magnetization and is highly susceptible to the strain, which is transmitted from the SrTiO(3) substrate. We outline a possible explanation of this unusual superconductivity-induced phenomenon in terms of a phase separation between ferromagnetic and non-ferromagnetic nanodomains in the La(2/3)Ca(1/3)MnO(3) layers.
人工多层膜为结合具有超导性和铁磁性等对抗性有序态的材料提供了独特机会,从而实现新型量子态。特别是,氧化物多层膜能够利用铜酸盐的高超导转变温度以及巨磁电阻锰氧化物的多种磁特性。然而,除了探索性工作外,对其异常特性的深入研究才刚刚开始。在此,我们展示了对Y(0.6)Pr(0.4)Ba(2)Cu(3)O(7)(10纳米)/La(2/3)Ca(1/3)MnO(3)(10纳米)超晶格的中子反射测量结果,这些结果揭示了超导性引起的垂直铁磁磁化分布的惊人调制。最令人惊讶的是,这种调制似乎涉及磁化强度的密度而非取向,并且对从SrTiO(3)衬底传递来的应变高度敏感。我们根据La(2/3)Ca(1/3)MnO(3)层中铁磁和非铁磁纳米域之间的相分离,概述了对这种异常超导诱导现象的一种可能解释。