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使用多周期驱动脉冲表征来自空心波导的孤立阿秒脉冲。

Characterizing isolated attosecond pulses from hollow-core waveguides using multi-cycle driving pulses.

作者信息

Thomann I, Bahabad A, Liu X, Trebino R, Murnane M M, Kapteyn H C

机构信息

JILA, University of Colorado and NIST, Boulder, Colorado 80309, USA.

出版信息

Opt Express. 2009 Mar 16;17(6):4611-33. doi: 10.1364/oe.17.004611.

Abstract

The generation of attosecond-duration light pulses using the high-order harmonic generation process is a rapidly evolving area of research. In this work, we combine experimental measurements with careful numerical analysis, to demonstrate that even relatively long-duration, 15 fs, carrier-envelope-phase (CEP) unstabilized near-infrared (NIR) pulses can generate isolated attosecond extreme-ultraviolet (EUV) pulses by the dynamically-changing phase matching conditions in a hollow-core waveguide geometry. The measurements are made using the laser-assisted photoelectric effect to cross-correlate the EUV pulse with the NIR pulse. A FROG CRAB analysis of the resulting traces (photoelectron signal versus photoelectron energy and EUV-NIR delay) is performed using a generalized projections (GP) algorithm, adapted for a wide-angle photoelectron detection geometry and non-CEP stabilized driving laser pulses. In addition, we performed direct FROG CRAB simulations under the same conditions. Such direct simulations allow more freedom to explore the effect of specific pulse parameters on FROG CRAB traces than is possible using the automated GP retrieval algorithm. Our analysis shows that an isolated pulse with duration of approximately 200 attoseconds can result from CEP unstabilized, high intensity approximately 15 fs multi-cycle driving pulses coupled into a hollow-core waveguide filled with low-pressure Argon gas. These are significantly longer driving pulses than used in other experimental implementations of isolated attosecond pulses.

摘要

利用高次谐波产生过程生成阿秒级持续时间的光脉冲是一个快速发展的研究领域。在这项工作中,我们将实验测量与细致的数值分析相结合,以证明即使是相对较长持续时间(15飞秒)、载波包络相位(CEP)不稳定的近红外(NIR)脉冲,也能通过空心波导几何结构中动态变化的相位匹配条件产生孤立的阿秒极紫外(EUV)脉冲。测量是利用激光辅助光电效应将EUV脉冲与NIR脉冲进行互相关来进行的。使用一种适用于广角光电子探测几何结构和非CEP稳定驱动激光脉冲的广义投影(GP)算法,对所得迹线(光电子信号与光电子能量及EUV - NIR延迟)进行频域相位分辨光电子能谱(FROG CRAB)分析。此外,我们在相同条件下进行了直接的FROG CRAB模拟。与使用自动GP检索算法相比,这种直接模拟在探索特定脉冲参数对FROG CRAB迹线的影响方面具有更大的自由度。我们的分析表明,CEP不稳定、高强度、约15飞秒的多周期驱动脉冲耦合到充满低压氩气的空心波导中,可以产生持续时间约为200阿秒的孤立脉冲。这些驱动脉冲比其他孤立阿秒脉冲的实验实现中所使用的脉冲长得多。

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