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利用空心毛细管光纤中的自压缩亚周期驱动实现稳健的孤立阿秒脉冲产生

Robust Isolated Attosecond Pulse Generation with Self-Compressed Subcycle Drivers from Hollow Capillary Fibers.

作者信息

Galán Marina Fernández, Serrano Javier, Jarque Enrique Conejero, Borrego-Varillas Rocío, Lucchini Matteo, Reduzzi Maurizio, Nisoli Mauro, Brahms Christian, Travers John C, Hernández-García Carlos, San Roman Julio

机构信息

Grupo de Investigación en Aplicaciones del Láser y Fotónica, Departamento de Física Aplicada, Universidad de Salamanca, Salamanca, 37008, Spain.

Unidad de Excelencia en Luz y Materia Estructuradas (LUMES), Universidad de Salamanca, Salamanca, 37008, Spain.

出版信息

ACS Photonics. 2024 Mar 18;11(4):1673-1683. doi: 10.1021/acsphotonics.3c01897. eCollection 2024 Apr 17.

Abstract

High-order harmonic generation (HHG) arising from the nonperturbative interaction of intense light fields with matter constitutes a well-established tabletop source of coherent extreme-ultraviolet and soft X-ray radiation, which is typically emitted as attosecond pulse trains. However, ultrafast applications increasingly demand isolated attosecond pulses (IAPs), which offer great promise for advancing precision control of electron dynamics. Yet, the direct generation of IAPs typically requires the synthesis of near-single-cycle intense driving fields, which is technologically challenging. In this work, we theoretically demonstrate a novel scheme for the straightforward and compact generation of IAPs from multicycle infrared drivers using hollow capillary fibers (HCFs). Starting from a standard, intense multicycle infrared pulse, a light transient is generated by extreme soliton self-compression in a HCF with decreasing pressure and is subsequently used to drive HHG in a gas target. Owing to the subcycle confinement of the HHG process, high-contrast IAPs are continuously emitted almost independently of the carrier-envelope phase (CEP) of the optimally self-compressed drivers. This results in a CEP-robust scheme which is also stable under macroscopic propagation of the high harmonics in a gas target. Our results open the way to a new generation of integrated all-fiber IAP sources, overcoming the efficiency limitations of usual gating techniques for multicycle drivers.

摘要

强激光场与物质的非微扰相互作用产生的高次谐波产生(HHG)构成了一种成熟的桌面型相干极紫外和软X射线辐射源,其通常以阿秒脉冲序列的形式发射。然而,超快应用越来越需要孤立阿秒脉冲(IAP),这为推进电子动力学的精确控制带来了巨大希望。然而,直接产生IAP通常需要合成近单周期强驱动场,这在技术上具有挑战性。在这项工作中,我们从理论上证明了一种新颖的方案,用于使用空心毛细管光纤(HCF)从多周期红外驱动源直接且紧凑地产生IAP。从一个标准的强多周期红外脉冲开始,在压力逐渐降低的HCF中通过极端孤子自压缩产生一个光瞬态,随后用于驱动气体靶中的HHG。由于HHG过程的亚周期限制,高对比度IAP几乎连续发射,几乎与最优自压缩驱动源的载波包络相位(CEP)无关。这导致了一种CEP鲁棒的方案,该方案在高次谐波在气体靶中的宏观传播下也是稳定的。我们的结果为新一代集成全光纤IAP源开辟了道路,克服了多周期驱动源常用选通技术的效率限制。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/0453/11027177/4ed8a2a2cc3c/ph3c01897_0001.jpg

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