Dufresne Eric M, Dierker Steven B, Yin Z, Berman Lonny
The Advanced Photon Source, Argonne National Laboratory, Argonne, IL 60439, USA.
J Synchrotron Radiat. 2009 May;16(Pt 3):358-67. doi: 10.1107/S0909049509003720. Epub 2009 Mar 20.
When one performs a coherent small-angle X-ray scattering experiment, the incident beam must be spatially filtered by slits on a length scale smaller than the transverse coherence length of the source which is typically around 10 microm. The Fraunhofer diffraction pattern of the slit is one of the important sources of background in these experiments. New slits which minimize this parasitic background have been designed and tested. The slit configuration apodizes the beam by the use of partially transmitting inclined slit jaws. A model is presented which predicts that the high wavevector tails of the diffraction pattern fall as the inverse fourth power of the wavevector instead of the inverse second power that is observed for standard slits. Using cleaved GaAs single-crystal edges, Fraunhofer diffraction patterns from 3 and 5.5 keV X-rays were measured, in agreement with the theoretical model proposed. A novel phase-peak diffraction pattern associated with phase variations of the transmitted electric field was also observed. The model proposed adequately accounts for this phenomenon.
当进行相干小角X射线散射实验时,入射光束必须通过狭缝在空间上进行滤波,狭缝的长度尺度要小于源的横向相干长度,该横向相干长度通常约为10微米。狭缝的夫琅禾费衍射图样是这些实验中背景的重要来源之一。已经设计并测试了能使这种寄生背景最小化的新型狭缝。这种狭缝配置通过使用部分透射的倾斜狭缝夹来对光束进行变迹处理。提出了一个模型,该模型预测衍射图样的高波矢尾部随波矢的四次方反比下降,而不是标准狭缝所观察到的二次方反比。使用解理的砷化镓单晶边缘,测量了3 keV和5.5 keV X射线的夫琅禾费衍射图样,与所提出的理论模型一致。还观察到了一种与透射电场的相位变化相关的新型相峰衍射图样。所提出的模型充分解释了这一现象。