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[江西相山铀矿田与非铀矿田水稻天然放射性核素含量对比研究]

[Contrast study on natural radioactive nuclides contents of rice between Xiangshan uranium deposit area, Jiangxi and non-uranium depsoit area].

作者信息

Liu Ping-Hui, Ye Chang-Sheng, Xie Shu-Rong, Rui Yu-Kui

机构信息

Key Laboratory of Nuclear Resources and Environment (East China Institute of Technology), Ministry of Education, Nanchang 330013, China.

出版信息

Guang Pu Xue Yu Guang Pu Fen Xi. 2009 Jul;29(7):1972-5.

Abstract

The contents of natural radioactive nuclides such as uranium and thorium in paddies were analyzed and compared by means of ICP-MS. Totally 14 paddy samples were distinguished into two groups and collected from two rice planting area. One group (12 paddy samples) was collected from the Xiangshan uranium deposit area, Jiangxi province; while the other group (2 samples) collected from non-uranium deposit suburban area of Fuzhou city, Jiangxi, as comparison samples. The distance between the two sampling areas is about 80 kilometers. Before analysis, those paddy samples were continuously carbonized by two hours first, then continuously incinerated for 8 hours at the temperature of 600 degrees centigrade. The results show that the uranium contents in the paddy ash of samples gotten from Xiangshan uranium deposit area range from 0.053 to 1.482 microg x g(-1). The uranium contents of two comparison paddy samples ash are 0.059 and 0.061 microg x g(-1), respectiovely. The average uranium content of paddy ash of uranium deposit area is 0.323 microg x g(-1). Compared with the comparison samples, the uranium contents of paddy ash of uranium deposit area are considerably high, 5.30 times that of non-uranium deposit area. The thorium contents in paddy ash of the uranium deposit area, however, are relatively low and less than that of samples collected from non-uranium deposit area, which range from 0.029 to 0.311 microg x g(-1); The average level is 0.104 microg x g(-1), only about 50% of that of paddy ash sampled from non-urnaium deposit area. Moreover, there is significant linearity correlation between uranium and thorium contents of paddy sampled from Xiangshan uranium deposit area. The positive effects show that the thorium contents of paddy increase as uranium contents of paddy in uranium deposit area increase. The causes for the remarkable difference in uranium contents in paddy between urianium deposit area and non-uranium deposit area are not clear yet. The research on this topic, however, is very important and significant to the regional rice quality and food security.

摘要

采用电感耦合等离子体质谱法(ICP-MS)对稻田中铀、钍等天然放射性核素的含量进行了分析和比较。从两个水稻种植区共采集了14个稻田样品,并分为两组。一组(12个稻田样品)采自江西省相山铀矿地区;另一组(2个样品)采自江西省抚州市非铀矿郊区作为对照样品。两个采样区之间的距离约为80公里。分析前,先将这些稻田样品连续碳化2小时,然后在600摄氏度的温度下连续焚烧8小时。结果表明,相山铀矿地区采集的样品的稻壳灰中铀含量在0.053至1.482μg·g⁻¹之间。两个对照稻田样品灰的铀含量分别为0.059和0.061μg·g⁻¹。铀矿地区稻田灰的平均铀含量为0.323μg·g⁻¹。与对照样品相比,铀矿地区稻田灰的铀含量相当高,是非铀矿地区的5.30倍。然而,铀矿地区稻田灰中的钍含量相对较低,低于非铀矿地区采集的样品,其范围在0.029至0.311μg·g⁻¹之间;平均水平为0.104μg·g⁻¹,仅为非铀矿地区稻田灰的约50%。此外,相山铀矿地区采集的稻田样品中铀和钍含量之间存在显著的线性相关。正效应表明,铀矿地区稻田中的钍含量随着铀含量的增加而增加。铀矿地区和非铀矿地区稻田中铀含量存在显著差异的原因尚不清楚。然而,对这一课题的研究对于区域水稻品质和粮食安全非常重要且意义重大。

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