Climate Research Group, School of Geography, Planning and Environmental Management, The University of Queensland, St Lucia, Brisbane, Qld 4072, Australia.
Environ Pollut. 2010 May;158(5):1615-28. doi: 10.1016/j.envpol.2009.12.009. Epub 2010 Jan 12.
Two peat bogs from remote alpine sites in Australia were found to contain detailed and coherent histories of atmospheric metal pollution for Pb, Zn, Cu, Mo, Ag, As, Cd, Sb, Zn, In, Cr, Ni, Tl and V. Dramatic increases in metal deposition in the post-1850 AD portion of the cores coincide with the onset of mining in Australia. Using both Pb isotopes and metals, pollutants were ascribed to the main atmospheric pollution emitting sources in Australia, namely mining and smelting, coal combustion and agriculture. Results imply mining and metal production are the major source of atmospheric metal pollution, although coal combustion may account for up to 30% of metal pollutants. A novel finding of this study is the increase in the otherwise near-constant Y/Ho ratio after 1900 AD. We link this change to widespread and increased application of marine phosphate fertiliser in Australia's main agricultural area (the Murray Darling Basin).
两个来自澳大利亚偏远高山地区的泥炭沼泽被发现含有详细而连贯的大气金属污染历史,包括 Pb、Zn、Cu、Mo、Ag、As、Cd、Sb、Zn、In、Cr、Ni、Tl 和 V。核心物质中后 1850 年部分的金属沉积急剧增加,与澳大利亚采矿的开始时间相吻合。利用 Pb 同位素和金属,将污染物归因于澳大利亚主要的大气污染排放源,即采矿和冶炼、煤炭燃烧和农业。结果表明,采矿和金属生产是大气金属污染的主要来源,尽管煤炭燃烧可能占金属污染物的 30%。本研究的一个新发现是,1900 年后,原本几乎不变的 Y/Ho 比值增加。我们将这一变化与澳大利亚主要农业区(墨累-达令盆地)中广泛且日益增加的海洋磷酸盐肥料的使用联系起来。