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个体暴露于超细颗粒物。

Personal exposure to ultrafine particles.

出版信息

J Expo Sci Environ Epidemiol. 2011 Jan-Feb;21(1):20-30. doi: 10.1038/jes.2009.59. Epub 2010 Jan 20.

Abstract

Personal exposure to ultrafine particles (UFP) can occur while people are cooking, driving, smoking, operating small appliances such as hair dryers, or eating out in restaurants. These exposures can often be higher than outdoor concentrations. For 3 years, portable monitors were employed in homes, cars, and restaurants. More than 300 measurement periods in several homes were documented, along with 25 h of driving two cars, and 22 visits to restaurants. Cooking on gas or electric stoves and electric toaster ovens was a major source of UFP, with peak personal exposures often exceeding 100,000 particles/cm³ and estimated emission rates in the neighborhood of 10¹² particles/min. Other common sources of high UFP exposures were cigarettes, a vented gas clothes dryer, an air popcorn popper, candles, an electric mixer, a toaster, a hair dryer, a curling iron, and a steam iron. Relatively low indoor UFP emissions were noted for a fireplace, several space heaters, and a laser printer. Driving resulted in moderate exposures averaging about 30,000 particles/cm³ in each of two cars driven on 17 trips on major highways on the East and West Coasts. Most of the restaurants visited maintained consistently high levels of 50,000-200,000 particles/cm³ for the entire length of the meal. The indoor/outdoor ratios of size-resolved UFP were much lower than for PM₂.₅ or PM₁₀, suggesting that outdoor UFP have difficulty in penetrating a home. This in turn implies that outdoor concentrations of UFP have only a moderate effect on personal exposures if indoor sources are present. A time-weighted scenario suggests that for typical suburban nonsmoker lifestyles, indoor sources provide about 47% and outdoor sources about 36% of total daily UFP exposure and in-vehicle exposures add the remainder (17%). However, the effect of one smoker in the home results in an overwhelming increase in the importance of indoor sources (77% of the total).

摘要

个人暴露于超细颗粒(UFP)可能发生在人们做饭、驾驶、吸烟、操作吹风机等小家电或在餐馆就餐时。这些暴露通常比户外浓度更高。在 3 年内,便携式监测器被用于家庭、汽车和餐馆。在多个家庭中记录了超过 300 个测量周期,同时还记录了 25 小时驾驶两辆汽车和 22 次到餐馆就餐的情况。使用煤气或电炉以及电烤面包炉烹饪是 UFP 的主要来源,个人暴露峰值通常超过 100000 个颗粒/cm³,估计排放率在 10¹² 个颗粒/分钟左右。其他高 UFP 暴露的常见来源是香烟、通风煤气烘干机、空气爆米花机、蜡烛、电动搅拌器、烤面包机、吹风机、卷发器和蒸汽熨斗。相对较低的室内 UFP 排放量被认为是壁炉、几个空间加热器和激光打印机。驾驶导致中等暴露,在东海岸和西海岸的主要高速公路上驾驶两辆汽车的 17 次旅行中,每辆车的平均暴露量约为 30000 个颗粒/cm³。大多数访问的餐厅在整个用餐过程中都保持着 50000-200000 个颗粒/cm³的持续高水平。按粒径分级的 UFP 的室内/室外比值远低于 PM₂.₅或 PM₁₀,这表明户外 UFP 很难穿透家庭。这反过来意味着,如果存在室内源,户外 UFP 浓度对个人暴露的影响只有中等程度。时间加权情景表明,对于典型的郊区非吸烟者生活方式,室内源提供了约 47%的总日 UFP 暴露和车辆内暴露的剩余部分(17%),而户外源提供了约 36%。然而,家中有一个吸烟者会导致室内源的重要性大大增加(占总数的 77%)。

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