Department of Chemistry, University of Sistan & Baluchestan, PO Box 98135-674, Zahedan, Iran.
J Comput Aided Mol Des. 2010 May;24(5):409-16. doi: 10.1007/s10822-010-9348-2. Epub 2010 Mar 30.
The substituent effects on the geometrical parameters and the individual hydrogen bond (HB) energies of base pairs such as X-adenine-thymine (X-A-T), X-thymine-adenine (X-T-A), X-guanine-cytosine (X-G-C), and X-cytosine-guanine (X-C-G) have been studied by the quantum mechanical calculations at the B3LYP and MP2 levels with the 6-311++G(d,p) basis set. The electron withdrawing (EW) substituents (F and NO(2)) increase the total binding energy (DeltaE) of X-G-C derivatives and the electron donating (ED) substituent (CH(3)) decreases it when they are introduced in the 8 and 9 positions of G. The effects of substituents are reversed when they are located in the 1, 5, and 6 positions of C, with exception of CH(3) in the 1 position and F in the 5 position, which in both cases the DeltaE value decreases negligibly small. With minor exceptions (X=8-CH(3), 8-F, and 9-NO(2)), both ED and EW substituents increase slightly the DeltaE values of X-A-T derivatives. The individual HB energies (E (HB)s) have been estimated using electron densities that calculated at the hydrogen bond critical points (HBCPs) by the atoms in molecules (AIM) method. Most of changes of individual HBs are in consistent with the ED/EW nature of substituents and the role of atoms entered H-bonding. The remarkable change is observed for NO(2) substituted derivative in each case.
采用 B3LYP 和 MP2 方法在 6-311++G(d,p)基组水平上研究了碱基对(如 X-腺嘌呤-胸腺嘧啶(X-A-T)、X-胸腺嘧啶-腺嘌呤(X-T-A)、X-鸟嘌呤-胞嘧啶(X-G-C)和 X-胞嘧啶-鸟嘌呤(X-C-G))中取代基对几何参数和各个氢键(HB)能的影响。当电子吸电子(EW)取代基(F 和 NO2)引入 G 的 8 位和 9 位时,X-G-C 衍生物的总结合能(ΔE)增加,而电子供体(ED)取代基(CH3)则降低了它。当取代基位于 C 的 1、5 和 6 位时,取代基的影响是相反的,除了 C 的 1 位上的 CH3 和 5 位上的 F,在这两种情况下,ΔE 值减小得可以忽略不计。除了 X=8-CH3、8-F 和 9-NO2 之外,ED 和 EW 取代基都略微增加了 X-A-T 衍生物的ΔE 值。氢键能(E(HB)s)是使用分子中原子(AIM)方法在氢键临界点(HBCP)处计算的电子密度来估计的。大多数氢键的变化与取代基的 ED/EW 性质和进入氢键的原子的作用一致。在每种情况下,NO2 取代的衍生物都观察到显著的变化。