Department of Physics, University of Ottawa, 150 Louis Pasteur, Ottawa, Ontario, Canada.
Opt Lett. 2010 Jun 15;35(12):1947-9. doi: 10.1364/OL.35.001947.
We demonstrate high-harmonic generation in H(2)O using 800 and 1300 nm laser pulses up to a maximum intensity of 5x10(14) W/cm(2). Under optimal phase-matching conditions, photon energies up to approximately 60 and approximately 87 eV are produced by using 800 and 1300 nm light, respectively. The harmonic spectra in H(2)O, when compared with Xe with a similar ionization potential, exhibit significant extension of the cutoff region, indicating suppression of ionization arising from molecular orbital symmetry.
我们使用 800nm 和 1300nm 激光脉冲在 H(2)O 中展示了高次谐波产生,最大强度达到 5x10(14) W/cm(2)。在最佳相位匹配条件下,分别使用 800nm 和 1300nm 光可产生高达约 60eV 和约 87eV 的光子能量。与具有相似电离势的 Xe 相比,H(2)O 中的谐波谱显示出截止区域的显著扩展,表明抑制了来自分子轨道对称性的电离。