Chemistry Department, Faculty of Science, El-Menoufia University, Shebin El-Kom, Egypt.
J Phys Chem A. 2010 Aug 5;114(30):7996-8002. doi: 10.1021/jp103397f.
Density functional theory (DFT)/BMK and CBS-QB3 ab initio calculations have been carried out to study the structures and energetics of unimolecular decomposition reactions of isopropyl butanoate (IPB, C(3)H(7)C(O)OCH(CH(3))(2)) as a model biofuel. The results show a good performance of the BMK method. Among seven different dissociation channels of IPB, formation of butanoic acid and propene via a six-membered ring transition state is the most favorable reaction. On the other hand, formation of lower esters is hindered by high-energy barriers and unlikely occurs except at elevated temperatures. Simple bond scission costs less energy than lower ester formation. A comparison with methyl and ethyl esters indicates faster decomposition of IPB. The changes in bond lengths along minimum energy paths are discussed.
密度泛函理论(DFT)/BMK 和 CBS-QB3 从头算计算被用来研究异丁酸异丙酯(IPB,C(3)H(7)C(O)OCH(CH(3))(2))作为一种生物燃料模型的分子分解反应的结构和能量学。结果表明 BMK 方法具有很好的性能。在 IPB 的七种不同的分解通道中,通过六元环过渡态形成丁酸和丙烯是最有利的反应。另一方面,形成低酯的反应由于高能垒而受到阻碍,除了在高温下,否则不太可能发生。简单的键断裂比形成低酯消耗的能量更少。与甲酯和乙酯的比较表明 IPB 的分解更快。还讨论了沿最低能量路径的键长变化。