School of the Earth Sciences and Resources, China University of Geosciences, No 29 Xueyuanlu Haidianqu, Beijing 100083, China.
J Hazard Mater. 2011 Jan 15;185(1):336-45. doi: 10.1016/j.jhazmat.2010.09.039. Epub 2010 Sep 18.
The temporal and spatial distribution of heavy metals (Cd, Hg, Pb, As and Cr) in Poyang Lake, the largest freshwater lake (3050 km(2)) in China, were studied based on the sedimentary profiles. For this purpose, eight sedimentary cores were selected which located at lake area, outfall of lake and the main branch rivers, respectively. High-resolution profiles with interval 2 cm were used for analyzing the concentration of metals, and the ages of them were determined by (210)Pb and (137)Cs isotopic dating. While studying the change of metals concentration with the age in profile, it is found that the concentration of them in sediments was influenced not only by the sources in history but also by the sediment types. Based on this detailed work, the inventory and burden of heavy metals per decade were estimated in lake area during the past 50 years. Significantly, rivers-contribution ratio per decade was estimated to distinguish each river's contribution of heavy metals into lake while river-flux in history and metals concentration in profiles were considered as calculating factors. So, our research provides a proof to well understand the sedimentary history and the inputting history of heavy metals from main rivers into an inland lake.
基于沉积岩芯剖面,研究了中国最大的淡水湖(3050 平方公里)鄱阳湖重金属(Cd、Hg、Pb、As 和 Cr)的时空分布。为此,分别在湖区、出湖口和主要支流河流选择了 8 个沉积岩芯。使用高分辨率 2cm 间隔的岩芯剖面来分析金属浓度,并用(210)Pb 和(137)Cs 同位素测年来确定年龄。在研究剖面中金属浓度随年龄的变化时,发现沉积物中金属浓度不仅受历史来源的影响,还受沉积类型的影响。在此详细工作的基础上,估算了过去 50 年来湖区每十年重金属的储量和负荷。值得注意的是,估计了每个十年河流的贡献比,以区分每条河流对重金属输入湖泊的贡献,同时考虑了历史上的河流流量和剖面中的金属浓度作为计算因素。因此,我们的研究为深入了解内陆湖泊重金属的沉积历史和主要河流的输入历史提供了证据。