Empa, Swiss Federal Laboratories for Materials Testing and Research, Überlandstrasse 129, CH-8600 Dübendorf, Switzerland.
Environ Sci Technol. 2011 Jan 1;45(1):203-8. doi: 10.1021/es1028052. Epub 2010 Nov 15.
After atmospheric deposition and storage in the ice, glaciers are temporary reservoirs of persistent organic pollutants (POPs). Recently, the hypothesis that melting glaciers represent secondary sources of these pollutants has been introduced by investigations of the historical trend of POPs in a dated sediment core from the proglacial Alpine Lake Oberaar. Here, the hypothesis is further confirmed by the comparison of sediment data gathered from two Alpine lakes with a glaciated and a nonglaciated hydrological catchment. The two lakes (Lake Engstlen and Lake Stein in the Bernese Alps in Switzerland) are situated only 8 km apart at similar altitude and in the same meteorological catchment. In the nonglacial lake sediment of Lake Engstlen, PCBs and DDT (polychlorinated biphenyls and dichlorodiphenyl trichloroethane) levels culminated with the historic usage of these chemicals some 30-50 years ago. In the glacial Lake Stein, this peak was followed by a reincrease in the 1990s, which goes along with the accelerated melting of the adjacent glacier. This study confirms the hypothesis of glaciers being a secondary source of these pollutants and is in accordance with the earlier findings in Lake Oberaar.
在经过大气沉降和在冰中储存之后,冰川成为持久性有机污染物(POPs)的临时储存库。最近,有研究对阿尔卑斯山前冰川湖 Oberaar 的定年沉积物核心中的持久性有机污染物的历史趋势进行了调查,提出了一个假设,即冰川融化是这些污染物的次生源。通过对具有冰川和无冰川水文流域的两个阿尔卑斯湖的沉积物数据进行比较,进一步证实了这一假设。这两个湖泊(瑞士伯尔尼阿尔卑斯山的恩格施泰伦湖和施泰因湖)仅相距 8 公里,海拔相似,位于同一气象流域。在无冰川的恩格施泰伦湖的沉积物中,PCBs 和滴滴涕(多氯联苯和滴滴涕)的水平达到了历史上这些化学物质使用的高峰期,大约在 30-50 年前。在有冰川的施泰因湖中,这个高峰期之后在 20 世纪 90 年代又出现了一个回升,这与附近冰川的加速融化相吻合。这项研究证实了冰川是这些污染物的次生源的假设,与之前在 Oberaar 湖的研究结果一致。