Vodungbo Boris, Barszczak Sardinha Anna, Gautier Julien, Lambert Guillaume, Valentin Constance, Lozano Magali, Iaquaniello Grégory, Delmotte Franck, Sebban Stéphane, Lüning Jan, Zeitoun Philippe
Laboratoire d'Optique Appliquée, ENSTA ParisTech-CNRS-cole polytechnique, Chemin de la Hunire, Palaiseau, France.
Opt Express. 2011 Feb 28;19(5):4346-56. doi: 10.1364/OE.19.004346.
We report the generation of circularly polarized high order harmonics in the extreme ultraviolet range (18-27 nm) from a linearly polarized infrared laser (40 fs, 0.25 TW) focused into a neon filled gas cell. To circularly polarize the initially linearly polarized harmonics we have implemented a four-reflector phase-shifter. Fully circularly polarized radiation has been obtained with an efficiency of a few percents, thus being significantly more efficient than currently demonstrated direct generation of elliptically polarized harmonics. This demonstration opens up new experimental capabilities based on high order harmonics, for example, in biology and materials science. The inherent femtosecond time resolution of high order harmonic generating table top laser sources renders these an ideal tool for the investigation of ultrafast magnetization dynamics now that the magnetic circular dichroism at the absorption M-edges of transition metals can be exploited.
我们报告了在聚焦于充满氖气的气室中的线性偏振红外激光(40飞秒,0.25太瓦)产生的极紫外范围(18 - 27纳米)内的圆偏振高次谐波。为了使最初的线性偏振谐波圆偏振,我们采用了一个四反射器移相器。已经获得了效率为百分之几的完全圆偏振辐射,因此比目前所展示的直接产生椭圆偏振谐波的效率显著更高。这一演示开启了基于高次谐波的新实验能力,例如在生物学和材料科学领域。由于可以利用过渡金属吸收M边处的磁圆二色性,高次谐波产生台式激光源固有的飞秒时间分辨率使其成为研究超快磁化动力学的理想工具。