Laboratoire d'Optique Appliquée, ENSTA ParisTech-CNRS UMR 7639-École polytechnique, Chemin de la Hunière, Palaiseau, France.
Nat Commun. 2012;3:999. doi: 10.1038/ncomms2007.
Femtosecond magnetization phenomena have been challenging our understanding for over a decade. Most experiments have relied on infrared femtosecond lasers, limiting the spatial resolution to a few micrometres. With the advent of femtosecond X-ray sources, nanometric resolution can now be reached, which matches key length scales in femtomagnetism such as the travelling length of excited 'hot' electrons on a femtosecond timescale. Here we study laser-induced ultrafast demagnetization in Co/Pd multilayer films, which, for the first time, achieves a spatial resolution better than 100 nm by using femtosecond soft X-ray pulses. This allows us to follow the femtosecond demagnetization process in a magnetic system consisting of alternating nanometric domains of opposite magnetization. No modification of the magnetic structure is observed, but, in comparison with uniformly magnetized systems of similar composition, we find a significantly faster demagnetization time. We argue that this may be caused by direct transfer of spin angular momentum between neighbouring domains.
飞秒磁现象已经困扰了我们十多年。大多数实验都依赖于红外飞秒激光,这将空间分辨率限制在几微米以内。随着飞秒 X 射线源的出现,现在可以达到纳米级分辨率,这与飞磁学中的关键长度尺度相匹配,例如在飞秒时间尺度上激发的“热”电子的传播长度。在这里,我们研究了Co/Pd多层膜中的激光诱导超快退磁,首次通过使用飞秒软 X 射线脉冲实现了优于 100nm 的空间分辨率。这使我们能够在由相反磁化的纳米级畴交替组成的磁系统中跟踪飞秒退磁过程。我们没有观察到磁结构的任何改变,但与具有相似成分的均匀磁化系统相比,我们发现退磁时间明显更快。我们认为这可能是由于相邻畴之间的自旋角动量直接传递所致。