Charalampous Georgios, Hardalupas Yannis
Mechanical Engineering Department, Imperial College London, London, UK.
Appl Opt. 2011 Mar 20;50(9):1197-209. doi: 10.1364/AO.50.001197.
The dependence of fluorescent and scattered light intensities from spherical droplets on droplet diameter was evaluated using Mie theory. The emphasis is on the evaluation of droplet sizing, based on the ratio of laser-induced fluorescence and scattered light intensities (LIF/Mie technique). A parametric study is presented, which includes the effects of scattering angle, the real part of the refractive index and the dye concentration in the liquid (determining the imaginary part of the refractive index). The assumption that the fluorescent and scattered light intensities are proportional to the volume and surface area of the droplets for accurate sizing measurements is not generally valid. More accurate sizing measurements can be performed with minimal dye concentration in the liquid and by collecting light at a scattering angle of 60° rather than the commonly used angle of 90°. Unfavorable to the sizing accuracy are oscillations of the scattered light intensity with droplet diameter that are profound at the sidescatter direction (90°) and for droplets with refractive indices around 1.4.
利用米氏理论评估了来自球形液滴的荧光和散射光强度对液滴直径的依赖性。重点在于基于激光诱导荧光与散射光强度之比(LIF/米氏技术)对液滴尺寸进行评估。本文进行了一项参数研究,其中包括散射角、折射率实部以及液体中染料浓度(决定折射率虚部)的影响。对于精确的尺寸测量而言,荧光和散射光强度与液滴体积和表面积成正比这一假设通常并不成立。在液体中使用最低染料浓度并在60°散射角而非常用的90°散射角收集光,可以进行更精确的尺寸测量。不利于尺寸测量精度的是,散射光强度随液滴直径的振荡在侧向散射方向(90°)以及对于折射率约为1.4的液滴时较为显著。