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InGaAs自组装量子点中激子的四波混频动力学

Four-wave mixing dynamics of excitons in InGaAs self-assembled quantum dots.

作者信息

Borri Paola, Langbein Wolfgang

机构信息

School of Biosciences, Cardiff University, Cardiff CF10 3TL, UK.

出版信息

J Phys Condens Matter. 2007 Jul 25;19(29):295201. doi: 10.1088/0953-8984/19/29/295201. Epub 2007 Jun 11.

DOI:10.1088/0953-8984/19/29/295201
PMID:21483053
Abstract

In this paper we summarize our experimental work on the dephasing of excitons in self-assembled InAs/GaAs quantum dots, measured using a sensitive four-wave mixing technique in heterodyne detection. Transient four-wave mixing is a powerful technique to measure not only exciton dephasing times but also fine-structure splitting energies and exciton-biexciton binding energies which are important physical parameters for the implementation of quantum dots as source of polarization-entangled photon pairs and in the design of quantum algorithms. The scope of this paper is to review and discuss, in the context of present theories and in comparison with other experiments in the literature, the most significant results of our study on a series of thermally annealed quantum dots exhibiting systematic differences in the excitonic recombination energies and quantum confinement potentials. We will highlight the main outcomes of these measurements and give a perspective in terms of open questions that still need to be investigated, possible new experiments and potential areas of interest.

摘要

在本文中,我们总结了关于自组装InAs/GaAs量子点中激子退相的实验工作,该工作采用外差检测中的灵敏四波混频技术进行测量。瞬态四波混频是一种强大的技术,不仅可以测量激子退相时间,还能测量精细结构分裂能和激子 - 双激子结合能,这些都是将量子点用作偏振纠缠光子对源以及量子算法设计中的重要物理参数。本文的范围是在当前理论背景下,与文献中的其他实验进行比较,回顾和讨论我们对一系列热退火量子点的研究中最显著的结果,这些量子点在激子复合能量和量子限制势方面呈现出系统差异。我们将突出这些测量的主要结果,并就仍需研究的开放性问题、可能的新实验以及潜在的感兴趣领域给出展望。

相似文献

1
Four-wave mixing dynamics of excitons in InGaAs self-assembled quantum dots.InGaAs自组装量子点中激子的四波混频动力学
J Phys Condens Matter. 2007 Jul 25;19(29):295201. doi: 10.1088/0953-8984/19/29/295201. Epub 2007 Jun 11.
2
Electrical control of the exciton-biexciton splitting in self-assembled InGaAs quantum dots.自组装 InGaAs 量子点中激子-双激子分裂的电控制。
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Transient coherent nonlinear spectroscopy of single quantum dots.单量子点的瞬态相干非线性光谱学
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引用本文的文献

1
Dephasing of InAs quantum dot -shell excitons studied using two-dimensional coherent spectroscopy.利用二维相干光谱研究砷化铟量子点壳层激子的退相
Phys Rev B. 2018 Nov;98(19). doi: 10.1103/PhysRevB.98.195304.
2
Coherent and Incoherent Coupling Dynamics between Neutral and Charged Excitons in Monolayer MoSe2.单层 MoSe2 中中性激子和带电激子的相干和非相干耦合动力学。
Nano Lett. 2016 Aug 10;16(8):5109-13. doi: 10.1021/acs.nanolett.6b02041. Epub 2016 Jul 22.
3
Engineering the spin-flip limited exciton dephasing in colloidal CdSe/CdS quantum dots.
在胶体 CdSe/CdS 量子点中工程自旋翻转限制激子退相。
ACS Nano. 2012 Jun 26;6(6):5227-33. doi: 10.1021/nn300992a. Epub 2012 May 15.
4
Long lifetimes of quantum-dot intersublevel transitions in the terahertz range.太赫兹范围内量子点子能级跃迁的长寿命
Nat Mater. 2009 Oct;8(10):803-7. doi: 10.1038/nmat2511. Epub 2009 Aug 16.