Division of Superconductivity and Magnetism, Faculty of Physics and Geosciences, University of Leipzig, Leipzig, Germany.
Nanotechnology. 2011 Jun 24;22(25):254025. doi: 10.1088/0957-4484/22/25/254025. Epub 2011 May 16.
La(0.7)Sr(0.3)MnO(3)-SrRuO(3) superlattices with and without nanometrically thin SrTiO(3), BaTiO(3) and Ba(0.7)Sr(0.3)TiO(3) interlayers were grown by pulsed laser deposition. Transmission electron microscopy studies showed coherent growth of La(0.7)Sr(0.3)MnO(3), SrRuO(3) and SrTiO(3) layers with atomically sharp interfaces, even if individual layers were as thin as one or two unit cells. In contrast, misfit dislocations and unit cell high interfacial steps were observed at the interfaces between BaTiO(3) and one of the ferromagnetic layers. The presence of the interlayers as well as these extended defects had a significant influence on the magnetic properties of the superlattices, especially on the antiferromagnetic interlayer exchange coupling between the La(0.7)Sr(0.3)MnO(3) and SrRuO(3) layers and the exchange biasing. Surprisingly, exchange biasing was found to increase with decreasing strength of the antiferromagnetic interlayer exchange coupling. This was explained by different magnetization reversal mechanisms acting in the regimes of strong and weak interlayer exchange coupling.
具有和不具有纳米级 SrTiO3、BaTiO3 和 Ba0.7Sr0.3TiO3 层的 La(0.7)Sr(0.3)MnO(3)-SrRuO(3) 超晶格通过脉冲激光沉积生长。透射电子显微镜研究表明,即使单个层的厚度只有一个或两个单元,La(0.7)Sr(0.3)MnO(3)、SrRuO(3) 和 SrTiO3 层也能以原子级的界面实现相干生长。相比之下,在 BaTiO3 和铁磁层之间的界面处观察到失配位错和单元晶格高界面台阶。这些层的存在以及这些扩展缺陷对超晶格的磁性有显著影响,特别是对 La(0.7)Sr(0.3)MnO(3) 和 SrRuO(3)层之间的反铁磁层间交换耦合和交换偏置的影响。令人惊讶的是,发现交换偏置随着反铁磁层间交换耦合强度的降低而增加。这可以通过在强和弱层间交换耦合区域中作用的不同磁化反转机制来解释。