Ragel F C, Plessis P de V du, Strydom A M
School of Physics, University of the Witwatersrand, Private Bag 3, PO WITS 2050, Johannesburg, South Africa. Physics Department, University of Johannesburg, PO Box 524, Aucklandpark 2006, South Africa.
J Phys Condens Matter. 2009 Jan 28;21(4):046008. doi: 10.1088/0953-8984/21/4/046008. Epub 2009 Jan 8.
Measurements of electrical resistivity (ρ(T)), magnetoresistivity (MR), magnetic susceptibility (χ(T)) and heat capacity (C(P)(T)) are presented for the (Ce(1-x)La(x))PtIn alloy system of which the CePtIn parent is a known dense Kondo compound that does not order magnetically down to 50 mK. χ(T) for alloys 0≤x≤0.8 exhibits Curie-Weiss behaviour. ρ(T) results indicate a transition from a dense Kondo behaviour for 0≤x≤0.2 to a single-ion Kondo region (0.3≤x≤0.8). The Kondo energy scale as given by T(K) values calculated from MR studies and by the temperature T(max)(ρ(mag)) where the magnetic contribution to ρ(T) exhibits a maximum value, is compared with theoretical models. It is shown that the experimental results not only depend on a volume effect as given by the compressible Kondo lattice model of Lavagna but in addition confirm the more complex behaviour recently presented by Burdin and Fulde for a Kondo alloy system in which the magnetic (Ce) and non-magnetic (La) atoms are distributed randomly. Non-Fermi-liquid behaviour is predicted by Burdin and Fulde at certain critical concentrations of the alloy system and experimental evidence for this is presented through χ(T), ρ(T) and C(P)(T) measurements.
本文给出了(Ce(1-x)La(x))PtIn合金体系的电阻率(ρ(T))、磁电阻率(MR)、磁化率(χ(T))和热容(C(P)(T))的测量结果。其中,母体CePtIn是一种已知的致密近藤化合物,在低至50 mK的温度下不会发生磁有序。对于0≤x≤0.8的合金,χ(T)表现出居里-外斯行为。ρ(T)的结果表明,从0≤x≤0.2的致密近藤行为转变为单离子近藤区域(0.3≤x≤0.8)。将由MR研究计算得到的T(K)值以及磁对ρ(T)贡献呈现最大值时的温度T(max)(ρ(mag))所给出的近藤能量标度与理论模型进行了比较。结果表明,实验结果不仅取决于Lavagna的可压缩近藤晶格模型所给出的体积效应,而且还证实了Burdin和Fulde最近提出的一种近藤合金体系更为复杂的行为,其中磁性(Ce)和非磁性(La)原子随机分布。Burdin和Fulde预测在合金体系的某些临界浓度下会出现非费米液体行为,并通过χ(T)、ρ(T)和C(P)(T)测量给出了相关实验证据。