Department of Atmospheric, Oceanic, and Space Sciences, University of Michigan, Ann Arbor, MI 48109, USA.
Proc Natl Acad Sci U S A. 2011 Aug 16;108(33):13404-8. doi: 10.1073/pnas.1018526108. Epub 2011 Aug 1.
Satellite-based estimates of the aerosol indirect effect (AIE) are consistently smaller than the estimates from global aerosol models, and, partly as a result of these differences, the assessment of this climate forcing includes large uncertainties. Satellite estimates typically use the present-day (PD) relationship between observed cloud drop number concentrations (N(c)) and aerosol optical depths (AODs) to determine the preindustrial (PI) values of N(c). These values are then used to determine the PD and PI cloud albedos and, thus, the effect of anthropogenic aerosols on top of the atmosphere radiative fluxes. Here, we use a model with realistic aerosol and cloud processes to show that empirical relationships for ln(N(c)) versus ln(AOD) derived from PD results do not represent the atmospheric perturbation caused by the addition of anthropogenic aerosols to the preindustrial atmosphere. As a result, the model estimates based on satellite methods of the AIE are between a factor of 3 to more than a factor of 6 smaller than model estimates based on actual PD and PI values for N(c). Using ln(N(c)) versus ln(AI) (Aerosol Index, or the optical depth times angstrom exponent) to estimate preindustrial values for N(c) provides estimates for N(c) and forcing that are closer to the values predicted by the model. Nevertheless, the AIE using ln(N(c)) versus ln(AI) may be substantially incorrect on a regional basis and may underestimate or overestimate the global average forcing by 25 to 35%.
卫星估算的气溶胶间接效应(AIE)通常小于全球气溶胶模型的估算值,而且由于这些差异,对这种气候强迫的评估存在很大的不确定性。卫星估算值通常使用观测到的云滴数浓度(N(c))和气溶胶光学深度(AOD)之间的当前(PD)关系来确定工业化前(PI)的 N(c) 值。然后,这些值用于确定 PD 和 PI 云反照率,从而确定人为气溶胶对大气辐射通量的影响。在这里,我们使用一个具有现实气溶胶和云过程的模型来表明,从 PD 结果得出的 ln(N(c))与 ln(AOD)的经验关系并不代表人为气溶胶添加到工业化前大气中引起的大气扰动。因此,基于卫星方法的 AIE 的模型估计值比基于实际 PD 和 PI 值的模型估计值小 3 到 6 倍。使用 ln(N(c))与 ln(AI)(气溶胶指数,即光学深度乘以 Ångström 指数)来估算工业化前 N(c)的值,可提供更接近模型预测值的 N(c)和强迫估计值。尽管如此,ln(N(c))与 ln(AI)的 AIE 在区域基础上可能存在重大错误,并且可能低估或高估全球平均强迫 25%至 35%。