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一维无序系统中小极化子跳跃电导率的场和温度依赖性。

Field and temperature dependence of the small polaron hopping electrical conductivity in 1D disordered systems.

作者信息

Triberis G P, Dimakogianni M

出版信息

J Phys Condens Matter. 2009 Sep 23;21(38):385406. doi: 10.1088/0953-8984/21/38/385406. Epub 2009 Aug 27.

Abstract

We investigate the effect of the electric field and the temperature on the electrical conductivity of one-dimensional disordered systems due to phonon assisted hopping of small polarons. The microscopic transport mechanism is treated within the framework of the generalized molecular crystal model and the Kubo formula, while percolation theoretical arguments lead to analytical expressions for the macroscopic behavior of the electrical conductivity at high (multi-phonon assisted hopping) and low (few-phonon assisted hopping) temperatures under the influence of moderate electric fields. The theoretical results are successfully applied to recent experimental findings for a wide temperature range and from low up to moderate electric fields. Comparison is made with other theories.

摘要

我们研究了电场和温度对一维无序系统电导率的影响,该影响源于小极化子的声子辅助跳跃。微观输运机制是在广义分子晶体模型和久保公式的框架内进行处理的,而渗流理论的观点则得出了在中等电场影响下,高(多声子辅助跳跃)、低(少数声子辅助跳跃)温度下电导率宏观行为的解析表达式。理论结果成功地应用于最近在很宽温度范围以及从低到中等电场下的实验发现。并与其他理论进行了比较。

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