Graduate School of Engineering Science, Osaka University, Osaka 560-8531, Japan.
Phys Rev Lett. 2011 Jul 22;107(4):047002. doi: 10.1103/PhysRevLett.107.047002. Epub 2011 Jul 19.
We report 75As nuclear quadrupole resonance studies on (Ca4Al2O(6-y))(Fe2As2) with T(c) = 27 K. Measurement of nuclear-spin-relaxation rate 1/T1 has revealed a significant development of two-dimensional antiferromagnetic spin fluctuations down to T(c) in association with the smallest As-Fe-As bond angle. Below T(c), the temperature dependence of 1/T1 without any trace of the coherence peak is well accounted for by a nodeless s(±)-wave multiple-gaps model. From the fact that its T(c) is comparable to T(c) = 28 K in the optimally doped LaFeAsO(1-y) in which antiferromagnetic spin fluctuations are not dominant, we remark that antiferromagnetic spin fluctuations are not a unique factor for enhancing T(c) among Fe-based superconductors, but a condition for optimizing superconductivity should be addressed from the lattice structure point of view.
我们报告了 75As 核四极共振研究(Ca4Al2O(6-y))(Fe2As2),其 T(c) = 27 K。核自旋弛豫率 1/T1 的测量揭示了二维反铁磁自旋波动的显著发展,直到与最小的 As-Fe-As 键角相关的 T(c)。在 T(c)以下,没有相干峰的 1/T1 的温度依赖性很好地由无节点 s(±)-波多间隙模型解释。由于其 T(c)与最佳掺杂的 LaFeAsO(1-y)中的 T(c) = 28 K 相当,而后者中反铁磁自旋波动不是主导因素,我们指出,反铁磁自旋波动并不是 Fe 基超导体中提高 T(c)的唯一因素,而是优化超导电性的条件应该从晶格结构的角度来考虑。