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强少周期激光脉冲作用下HeH²⁺解离过程中电子局域化的相位依赖性

Phase dependence of electron localization in HeH²⁺ dissociation with an intense few-cycle laser pulse.

作者信息

Liu Kunlong, Hong Weiyi, Lu Peixiang

机构信息

Wuhan National Laboratory for Optoelectronics, Huazhong University of Science and Technology, Wuhan 430074, China.

出版信息

Opt Express. 2011 Oct 10;19(21):20279-87. doi: 10.1364/OE.19.020279.

Abstract

The electron localization in the dissociation of the asymmetric charged molecular ion HeH²⁺ exposed to an intense few-cycle laser pulse is studied by solving numerically the 3D time-dependent Schrödinger equation. By varying the carrier-envelope phase (CEP) and the intensity of the pulse, the upward shift of the localization probability and the suppression of the dissociation channel He²⁺+H are observed. Our analysis shows that the phenomenon is attributed to the asymmetric structure of the molecule as well as the recollision-assistant field-induced ionization of the electron wave packets localized on H⁺ in the trailing of the pulse.

摘要

通过数值求解三维含时薛定谔方程,研究了暴露于强少周期激光脉冲下的不对称带电分子离子HeH²⁺解离过程中的电子局域化。通过改变载波包络相位(CEP)和脉冲强度,观察到局域化概率的上移以及解离通道He²⁺+H的抑制。我们的分析表明,该现象归因于分子的不对称结构以及脉冲尾部局域在H⁺上的电子波包的再碰撞辅助场致电离。

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