Nuclear reaction induced by carrier-envelope-phase controlled proton recollision in a laser-driven molecule.

Nuclear reactions induced by proton recollision with a nearby nucleus are studied in a setup where a neutral molecule is exposed to an extremely intense, few-cycle laser pulse. At the rising edge of the laser pulse, all electrons in the molecule are first ejected by field ionization, resulting in a molecule consisting of the bare nuclei only. A proton in the bare molecule is subsequently accelerated by the laser field in such a way that it recollides with a nearby, heavier nucleus, with a kinetic energy high enough to induce a nuclear reaction. As a specific example, the probability of triggering the (15)N(p,α)(12)C reaction by exposing either a (15)NH molecule or a (15)NH3 molecule to an intense laser pulse is calculated using the classical trajectory Monte Carlo method. We show that the proton recollision process can be controlled both by varying the carrier-envelope phase of the laser field and by the degree of molecular orientation. We also find that the magnetic field of the laser pulse plays a crucial role in the recollision dynamics.