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在西伯利亚化学联合企业排放物影响下的托姆河和奥比河的长寿命人工放射性核素的最新浓度。

Up-to-date concentrations of long-lived artificial radionuclides in the Tom and Ob rivers in the area influenced by discharges from Siberian chemical combine.

机构信息

SI RPA Typhoon of Roshydromet, Pobeda Street 4, Obninsk Kaluga Region 249038, Russia.

出版信息

J Environ Radioact. 2012 Jun;108:15-23. doi: 10.1016/j.jenvrad.2011.11.013. Epub 2011 Dec 6.

DOI:10.1016/j.jenvrad.2011.11.013
PMID:22153591
Abstract

The Siberian Chemical Combine (SCC) is located in Seversk (formerly known as Tomsk-7) in the Tomsk Region of the Russian Federation. The main contribution of radionuclides in the SCC process water discharged into the Tom River was from the single-pass reactors, now removed from service (the last SCC reactor was shutdown on June 5, 2008). The data on the concentrations of (90)Sr, (137)Cs, (239,240)Pu and other artificial radionuclides in water, bottom sediments and flood-plain soils of the Tom and Ob rivers from Tomsk to the confluence of the rivers, are presented and discussed. The results of measurements carried out after shutdown of the last SCC single-pass reactor indicated no radiologically significant consequences of SCC activities for the studied water environment compartments. Contemporary activity concentrations of long-lived artificial radionuclides (3)H, (90)Sr, (137)Cs and (239,240)Pu in river water were below the intervention levels established by current regulations of the Russian Federation for these radionuclides. The results of (3)H analysis in water from the Tom and Samuska rivers demonstrated no inflow of contaminated formation water to surface water from the sites where liquid radioactive wastes of the SCC were injected below the surface. However, the density of flood-plain soil contamination by long-lived (137)Cs in the area influenced by SCC liquid discharges was higher than regional technogenic background. There were local flood-plain areas contaminated not only by (137)Cs, but also other gamma-emitters, such as (60)Co and (152)Eu.

摘要

西伯利亚化学联合企业(SCC)位于俄罗斯联邦托木斯克州的斯韦尔斯克(原名托木斯克-7)。SCC 工艺排放到托姆河中的过程水中放射性核素的主要贡献来自现已退役的单程反应器(最后一个 SCC 反应堆于 2008 年 6 月 5 日关闭)。本文提供并讨论了托姆河和额尔齐斯河从托木斯克到两河汇流处的河水、底泥和泛滥平原土壤中(90)Sr、(137)Cs、(239,240)Pu 等人工放射性核素的浓度数据。最后一个 SCC 单程反应器关闭后的测量结果表明,SCC 活动对所研究的水生态环境没有产生重大的放射性后果。在河水、底泥和泛滥平原土壤中,长寿命人工放射性核素(3)H、(90)Sr、(137)Cs 和(239,240)Pu 的当代活度浓度均低于俄罗斯联邦现行法规为这些核素规定的干预水平。托姆河和萨姆斯卡河水中(3)H 的分析结果表明,从 SCC 注入地下的放射性废液注入区没有受污染的地层水流入地表水。然而,在 SCC 液体排放物影响的泛滥平原土壤中,长寿命(137)Cs 的污染密度高于区域人为背景。有些泛滥平原地区不仅受到(137)Cs 的污染,还受到其他伽马放射性核素(如(60)Co 和(152)Eu)的污染。

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