School of Earth and Environmental Sciences, Queens College, and Graduate School and University Center, City University of New York, Flushing, New York 11367, United States.
Environ Sci Technol. 2012 Feb 7;46(3):1388-95. doi: 10.1021/es2032967. Epub 2012 Jan 17.
To understand redox-dependent arsenic partitioning, we performed batch sorption and desorption experiments using aquifer sands subjected to chemical and mineralogical characterization. Sands collected from the redox transition zone between reducing groundwater and oxic river water at the Meghna riverbank with HCl extractable Fe(III)/Fe ratio ranging from 0.32 to 0.74 are representative of the redox conditions of aquifers common in nature. One brown suboxic sediment displayed a partitioning coefficient (K(d)) of 7-8 L kg(-1) at equilibrium with 100 μg L(-1) As(III), while two gray reducing sediments showed K(d) of 1-2 L kg(-1). Lactate amendment to aquifer sands containing 91 mg kg(-1) P-extractable As resulted in the reduction of As and Fe with sediment Fe(III)/Fe decreasing from 0.54 to 0.44, and mobilized an equivalent of 64 mg kg(-1) As over a month. Desorption of As from nonlactate-amended sediment was negligible with little change in sediment Fe(III)/Fe. This release of As is consistent with microbial reduction of Fe(III) oxyhydroxides and the resulting decrease in the number of surface sites on Fe(III) oxyhydroxides. Arsenic partitioning (K(d)) in iron-rich, sulfur-poor aquifers with circumneutral pH is redox-dependent and can be estimated by HCl leachable sediment Fe(III)/Fe ratio with typical Fe concentrations.
为了理解氧化还原依赖的砷分配,我们使用经过化学和矿物学特征描述的含水层砂进行了批量吸附和解吸实验。从恒河河岸的还原地下水和氧化河水之间的氧化还原过渡带采集的砂,其 HCl 可提取 Fe(III)/Fe 比值范围为 0.32 至 0.74,代表了自然界中常见的含水层的氧化还原条件。一个棕色亚缺氧沉积物在与 100μg/L 的 As(III) 达到平衡时的分配系数(K(d))为 7-8 L/kg,而两个灰色还原沉积物的 K(d)为 1-2 L/kg。向含有 91mg/kg P 可提取砷的含水层砂中添加乳酸导致砷和铁的还原,沉积物 Fe(III)/Fe 从 0.54 降低至 0.44,并且在一个月内迁移了相当于 64mg/kg 的砷。未添加乳酸的沉积物中砷的解吸可以忽略不计,沉积物 Fe(III)/Fe 几乎没有变化。这种砷的释放与 Fe(III)氢氧化物的微生物还原一致,导致 Fe(III)氢氧化物表面位点数量减少。在 pH 值接近中性、富铁、贫硫的含水层中,砷的分配(K(d))是氧化还原依赖的,可以通过 HCl 可提取沉积物 Fe(III)/Fe 比值和典型的 Fe 浓度来估计。