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圆二色性在激光辅助短脉冲光致电离中的应用。

Circular dichroism in laser-assisted short-pulse photoionization.

机构信息

Departamento de Fisica de Materiales, UPV/EHU, E-20018 San Sebastian/Donostia, Spain.

出版信息

Phys Rev Lett. 2011 Dec 16;107(25):253002. doi: 10.1103/PhysRevLett.107.253002. Epub 2011 Dec 14.

Abstract

A remarkable effect of circular dichroism, i.e., a difference in photoelectron spectra produced by right and left circularly polarized light in two-color multiphoton ionization of atoms, is predicted for the case when the atom is ionized by an extreme ultraviolet or x-ray femtosecond pulse in the field of a strong infrared laser pulse, both pulses being circularly polarized. We show that the sidebands formed in the spectra exhibit different circular dichroism often of different signs both in angle-resolved and angle-integrated experimental conditions. The effect can be used for detecting and measuring circular polarization of x rays in a spectral range where other methods are not effective.

摘要

圆二色性的一个显著效应,即在原子双色多光子电离过程中,用圆偏振的极端紫外或 X 射线飞秒脉冲与强红外激光脉冲作用,左右圆偏振光产生的光电子能谱的差异,被预言。我们表明,在角分辨和角积分实验条件下,谱中形成的边带表现出不同的圆二色性,通常符号也不同。该效应可用于探测和测量在其他方法无效的光谱范围内 X 射线的圆偏振。

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