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利用旋转激光捕获微粒测量溶致液晶的粘度

Measurement of viscosity of lyotropic liquid crystals by means of rotating laser-trapped microparticles.

作者信息

Liu Qingkun, Asavei Theodor, Lee Taewoo, Rubinsztein-Dunlop Halina, He Sailing, Smalyukh Ivan I

机构信息

Department of Physics, University of Colorado, Boulder, CO 80309, USA.

出版信息

Opt Express. 2011 Dec 5;19(25):25134-43. doi: 10.1364/OE.19.025134.

Abstract

We describe a simple microrheology method to measure the viscosity coefficients of lyotropic liquid crystals. This approach is based on the use of a rotating laser-trapped optically anisotropic microsphere. In aligned liquid crystals that have negligible effect on trapping beam's polarization, the optical torque is transferred from circularly polarized laser trapping beam to the optically anisotropic microparticle and creates the shear flow in the liquid crystalline fluid. The balance of optical and viscous torques yields the local effective viscosity coefficients of the studied lyotropic systems in cholesteric and lamellar phases. This simple yet powerful method is capable of probing viscosity of complex anisotropic fluids for small amounts of sample and even in the presence of defects that obstruct the use of conventional rheology techniques.

摘要

我们描述了一种用于测量溶致液晶粘度系数的简单微观流变学方法。该方法基于使用旋转的激光捕获光学各向异性微球。在对捕获光束偏振影响可忽略不计的取向液晶中,光学扭矩从圆偏振激光捕获光束传递到光学各向异性微粒,并在液晶流体中产生剪切流。光学扭矩和粘性扭矩的平衡得出了所研究的胆甾相和层状相溶致体系的局部有效粘度系数。这种简单却强大的方法能够在只需少量样品的情况下,甚至在存在妨碍使用传统流变学技术的缺陷时,探测复杂各向异性流体的粘度。

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