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剪切流中软弹性粒子的形状动力学和流变学。

Shape dynamics and rheology of soft elastic particles in a shear flow.

机构信息

Department of Mechanical Engineering and Applied Mechanics, University of Pennsylvania, Philadelphia, Pennsylvania 19104, USA.

出版信息

Phys Rev Lett. 2012 Feb 3;108(5):058302. doi: 10.1103/PhysRevLett.108.058302. Epub 2012 Jan 31.

DOI:10.1103/PhysRevLett.108.058302
PMID:22400968
Abstract

The shape dynamics of soft, elastic particles in an unbounded simple shear flow is investigated theoretically under Stokes flow conditions. Three types of motion-steady-state, trembling, and tumbling-are predicted, depending on the shear rate, elastic shear modulus, and initial particle shape. The steady-state motion is found to be always stable. In addition, the existence of a trembling regime is documented for the first time in nonvesicle systems, and a complete phase diagram is developed. The rheological properties of dilute suspensions of such soft particles generally exhibit shear-thinning behavior and can even display negative intrinsic viscosity for sufficiently soft particles.

摘要

在无界简单剪切流中,研究了软弹性粒子在斯托克斯流条件下的形状动力学。根据剪切速率、弹性剪切模量和初始粒子形状,预测了三种运动状态:稳态、颤动和翻滚。发现稳态运动始终稳定。此外,首次在非囊泡系统中记录到颤动状态,并开发了完整的相图。这种软粒子稀悬浮液的流变性质通常表现出剪切变稀行为,对于足够软的粒子甚至可以表现出负的固有粘度。

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