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使用低频交流电润湿实现固着液滴在微倾斜平面上的尺寸选择性滑动。

Size-selective sliding of sessile drops on a slightly inclined plane using low-frequency AC electrowetting.

机构信息

Department of Mechanical Engineering, Pohang University of Science and Technology, San 31, Hyoja-dong, Pohang 790-784, South Korea.

出版信息

Langmuir. 2012 Apr 17;28(15):6307-12. doi: 10.1021/la2039703. Epub 2012 Apr 2.

Abstract

When placed on an inclined solid plane, drops often stick to the solid surface due to pinning forces caused by contact angle hysteresis. When the drop size or the plane's incline angle is small, the drop is difficult to slide due to a decrease in gravitational force. Here we demonstrate that small drops (0.4-9 μL) on a slightly inclined plane (~12°, Teflon and parylene-C surface) can be mobilized through patterned electrodes by applying low-frequency ac electrowetting under 400 Hz (110-180 V(rms)), which has a mechanism different from that of the high-frequency ac method that induces sliding by reducing contact angle hysteresis. We attribute the sliding motion of our method to a combination of contact angle hysteresis and interfacial oscillation driven by ac electrowetting instead of the minimization of contact angle hysteresis at a high frequency. We investigated the effects of ac frequency on the sliding motion and terminal sliding of drops; the terminal sliding velocity is greatest at resonance frequency. Varying the electrowetting number (0.21-0.56) at a fixed frequency (40 Hz) for 5 μL drops, we found an empirical relationship between the electrowetting number and the terminal sliding velocity. Using the relationship between the drop size and ac frequency, we can selectively slide drops of a specific size or merge two drops along an inclined plane. This simple method will help with constructing microfluidic platforms with sorting, merging, transporting, and mixing of drops without a programmable control of electrical signals. Also, this method has a potential in heat transfer applications because heat removal capacity can be enhanced significantly through drop oscillation.

摘要

当放置在倾斜的固体平面上时,由于接触角滞后引起的钉扎力,液滴通常会粘在固体表面上。当液滴尺寸或平面倾斜角度较小时,由于重力的减小,液滴很难滑动。在这里,我们展示了在略微倾斜的平面(~12°,特氟龙和派瑞林-C 表面)上的小液滴(0.4-9 μL)可以通过施加低频交流电润湿来通过图案化电极来移动,施加频率在 400 Hz 以下(110-180 V(rms)),其机制与通过减小接触角滞后来诱导滑动的高频交流电方法不同。我们将我们的方法的滑动运动归因于交流电润湿引起的接触角滞后和界面振荡的组合,而不是高频下接触角滞后的最小化。我们研究了交流电频率对液滴滑动和终端滑动的影响;在共振频率下,终端滑动速度最大。在固定频率(40 Hz)下,对于 5 μL 的液滴,改变电润湿数(0.21-0.56),我们发现电润湿数和终端滑动速度之间存在经验关系。使用液滴尺寸和交流电频率之间的关系,我们可以沿倾斜平面选择性地滑动特定尺寸的液滴或合并两个液滴。这种简单的方法将有助于构建具有排序、合并、输送和混合液滴的微流控平台,而无需可编程的电信号控制。此外,这种方法在传热应用中具有潜力,因为通过液滴振荡可以显著增强散热能力。

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