Chen Shunli, Zhao Yuan'an, Li Dawei, He Hongbo, Shao Jianda
Key Laboratory of Materials for High Power Laser, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai, China.
Appl Opt. 2012 Apr 1;51(10):1495-502. doi: 10.1364/AO.51.001495.
The effect of nanosecond laser pre-irradiation on the femtosecond laser-induced damage behaviors of 800 nm 0° AOI Ta(2)O(5)/SiO(2) high reflectors fabricated by e-beam evaporation was explored. Laser pre-irradiation was carried out by Raster-scanning with scanning mode of 1-on-1 and scanning velocities timed such that there was a beam overlap at 70% of the peak fluence, utilizing 5 Hz 1064 nm 12 ns Nd:YAG fundamental lasers. Femtosecond laser damage was investigated by 1 kHz 800 nm 135 fs Ti: sapphire laser system with 1-on-1 mode test. The results indicated that nanosecond laser pre-irradiation did not promote the femtosecond laser-induced damage threshold of reflectors. Instead, the thresholds of all the samples with various fluence steps for pre-irradiation were reduced by about 20%. Furthermore, the damage morphologies were analyzed by optical microscope, SEM and AFM, which displayed deterministic field induced breakdown characteristics. To explain these phenomena, a theoretical model including photoionization, avalanche ionization, and decays of electrons was built to simulate the evolution of electron density in the conduction band. Field ionization mechanism was considered to dominate the femtosecond laser damage process, while the electronic defects induced by nanosecond laser pre-irradiation accelerated the femtosecond laser damage evolution.
研究了纳秒激光预辐照对电子束蒸发制备的800 nm 0°入射角Ta₂O₅/SiO₂高反射镜飞秒激光诱导损伤行为的影响。采用5 Hz 1064 nm 12 ns Nd:YAG基频激光器,以1对1的扫描模式进行光栅扫描,设置扫描速度,使光束在峰值能量密度的70%处重叠,从而实现激光预辐照。利用1 kHz 800 nm 135 fs钛宝石激光系统,采用1对1模式测试来研究飞秒激光损伤。结果表明,纳秒激光预辐照并未提高反射镜的飞秒激光诱导损伤阈值。相反,所有不同预辐照能量密度步长的样品的阈值都降低了约20%。此外,通过光学显微镜、扫描电子显微镜和原子力显微镜对损伤形貌进行了分析,这些形貌呈现出确定性的场致击穿特征。为了解释这些现象,建立了一个包括光电离、雪崩电离和电子衰减的理论模型,以模拟导带中电子密度的演化。场电离机制被认为主导了飞秒激光损伤过程,而纳秒激光预辐照诱导的电子缺陷加速了飞秒激光损伤的演化。