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宽频单向散射的磁电核壳纳米粒子。

Broadband unidirectional scattering by magneto-electric core-shell nanoparticles.

机构信息

Nonlinear Physics Centre, Centre for Ultrahigh-Bandwidth Devices for Optical Systems (CUDOS), Research School of Physics and Engineering, Australian National University, Canberra, ACT 0200, Australia.

出版信息

ACS Nano. 2012 Jun 26;6(6):5489-97. doi: 10.1021/nn301398a. Epub 2012 May 4.

Abstract

Core-shell nanoparticles have attracted surging interests due to their flexibly tunable resonances and various applications in medical diagnostics, biosensing, nanolasers, and many other fields. The core-shell nanoparticles can support simultaneously both electric and magnetic resonances, and when the resonances are properly engineered, entirely new properties can be achieved. Here we study core-shell nanoparticles that support both electric and artificial magnetic dipolar modes, which are engineered to coincide spectrally with the same strength. We reveal that the interferences of these two resonances result in azimuthally symmetric unidirectional scattering, which can be further improved by arranging the nanoparticles in a chain, with both azimuthal symmetry and vanishing backward scattering preserved over a wide spectral range. We also demonstrate that the vanishing backward scattering is preserved, even for random particle distributions, which can find applications in the fields of nanoantennas, photovoltaic devices, and nanoscale lasers that require backward scattering suppressions.

摘要

核壳纳米粒子由于其可调谐的共振和在医学诊断、生物传感、纳米激光等诸多领域的各种应用而引起了人们的浓厚兴趣。核壳纳米粒子可以同时支持电共振和磁共振,并且当这些共振被合理设计时,可以获得全新的性质。在这里,我们研究了同时支持电共振和人工磁偶极共振的核壳纳米粒子,这两种共振被设计为在相同的强度下实现光谱匹配。我们揭示了这两种共振的相互干扰导致了各向同性的单向散射,通过将纳米粒子排列成链状,可以进一步改善这种散射,并且在很宽的光谱范围内保持各向同性和零后向散射。我们还证明了即使在随机粒子分布的情况下,零后向散射也可以得到保持,这在需要抑制后向散射的纳米天线、光伏器件和纳米尺度激光等领域都有应用。

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