Graduate School of Science and Engineering, Saitama University, 255 Shimo-Okubo, Sakura-ku, Saitama 338-8570, Japan.
Sensors (Basel). 2012;12(5):5420-31. doi: 10.3390/s120505420. Epub 2012 Apr 27.
Fluorescence sensing of saccharides and glycoproteins using a boronic acid functionalized squarylium cyanine dye ("SQ-BA") is characterized in terms of synthetic, fluorometric, thermodynamic and kinetic parameters. In our previous work, this newly synthesized dye was successfully applied to the separation and quantification of Gram-positive bacteria by capillary electrophoresis with laser-induced fluorescence detection (CE-LIF); however, the fundamental properties of the dye and its saccharide complexes still required elucidation, as presented in this paper. The dye itself forms nonemissive, soluble aggregates in aqueous solution. With the addition of a monosaccharide, the dye aggregate dissociates to form an emissive monomer accompanied by the formation of a cyclic cis-diol ester with long-wavelength emission (λ(ex) = 630 nm, λ(em) = 660 nm). A very large fluorescence enhancement factor of 18× was observed for the sensing dye as a fructose complex at pH 10, yielding a limit of detection of 10 μM fructose. The relative order of fluorescence enhancement of SQ-BA with other monosaccharides was found to be: fructose > ribose > arabinose ≈ galactose > xylose > mannose > rhamnose > fucose ≈ glucose; and apparent affinity constants of 10(2.80), 10(2.08) and 10(0.86) M(-1) were determined for fructose, ribose and glucose, respectively. Formation of the emissive complexes occurred within minutes, proving the kinetics of the sugar-dye interactions to be suitable for on-column labeling methods in CE-LIF. Furthermore, the sensing dye was successfully applied to glycoproteins, mucin type I-S and type III, which were detected with high sensitivity in batch aqueous solution as a result of the sugar-selective boronic acid-diol esterification as well as hydrophobic interactions.
使用硼酸功能化方酸菁染料(“SQ-BA”)对糖和糖蛋白进行荧光传感,从合成、荧光、热力学和动力学参数方面进行了描述。在我们之前的工作中,这种新合成的染料已成功应用于通过激光诱导荧光检测的毛细管电泳(CE-LIF)对革兰氏阳性细菌的分离和定量;然而,正如本文所述,该染料及其糖复合物的基本性质仍需要阐明。染料本身在水溶液中形成非发光、可溶的聚集体。加入单糖后,染料聚集体解离形成发光单体,同时形成具有长波长发射的环状顺式二醇酯(λ(ex) = 630nm,λ(em) = 660nm)。在 pH 10 下,作为果糖复合物,传感染料的荧光增强因子非常大,达到 18×,果糖的检测限为 10μM。发现 SQ-BA 与其他单糖的荧光增强相对顺序为:果糖 > 核糖 > 阿拉伯糖≈半乳糖 > 木糖 > 甘露糖 > 鼠李糖 > 岩藻糖≈葡萄糖;并且分别确定了果糖、核糖和葡萄糖的表观亲和力常数为 10(2.80)、10(2.08)和 10(0.86)M(-1)。发射性复合物的形成在数分钟内发生,证明糖-染料相互作用的动力学适合 CE-LIF 中的柱上标记方法。此外,传感染料成功地应用于糖蛋白、I-S 型和 III 型粘蛋白,由于糖选择性硼酸-二醇酯化以及疏水相互作用,在批处理水溶液中具有高灵敏度。