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二维空间中孤立对的可逆扩散影响反应的精确格林函数。

Exact Green's function of the reversible diffusion-influenced reaction for an isolated pair in two dimensions.

机构信息

Laboratory of Systems Biology, National Institute of Allergy and Infectious Diseases, National Institutes of Health, Bethesda, Maryland 20892, USA.

出版信息

J Chem Phys. 2012 Aug 7;137(5):054104. doi: 10.1063/1.4737662.

DOI:10.1063/1.4737662
PMID:22894329
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC3422329/
Abstract

We derive an exact Green's function of the diffusion equation for a pair of disk-shaped interacting particles in two dimensions subject to a backreaction boundary condition. Furthermore, we use the obtained function to calculate exact expressions for the survival probability and the time-dependent rate coefficient for the initially unbound pair and the survival probability of the bound state. The derived expressions will be of particular utility for the description of reversible membrane-bound reactions in cell biology.

摘要

我们推导出了一个在二维空间中,受到反作用边界条件约束的一对相互作用的圆盘状粒子的扩散方程的精确格林函数。此外,我们还使用所得到的函数来计算初始未结合对的生存概率和时变速率系数以及结合态的生存概率的精确表达式。所推导的表达式对于描述细胞生物学中可逆的膜结合反应将特别有用。

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引用本文的文献

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Diffusion in a disk with inclusion: Evaluating Green's functions.含夹杂圆盘内的扩散:格林函数评估
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Space-time histories approach to fast stochastic simulation of bimolecular reactions.时空历史方法快速随机模拟双分子反应。
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Quantifying the roles of space and stochasticity in computer simulations for cell biology and cellular biochemistry.量化空间和随机性在细胞生物学和细胞生物化学计算机模拟中的作用。
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Unified path integral approach to theories of diffusion-influenced reactions.扩散影响反应理论的统一路径积分方法。
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Theory of bi-molecular association dynamics in 2D for accurate model and experimental parameterization of binding rates.二维双分子缔合动力学理论,用于结合速率的精确模型和实验参数化。
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7
The area reactivity model of geminate recombination.孪生复合的区域反应性模型。
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8
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J Chem Phys. 2013 Nov 21;139(19):194103. doi: 10.1063/1.4830218.
9
Theory of reversible diffusion-influenced reactions with non-Markovian dissociation in two space dimensions.二维空间中非马尔可夫解吸的可逆扩散反应理论。
J Chem Phys. 2013 Mar 14;138(10):104112. doi: 10.1063/1.4794311.

本文引用的文献

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Spatial organization of transmembrane receptor signalling.跨膜受体信号的空间组织。
EMBO J. 2010 Aug 18;29(16):2677-88. doi: 10.1038/emboj.2010.175.
2
Excited-state reversible geminate recombination in two dimensions.二维激发态可逆孪生复合
J Chem Phys. 2009 Oct 21;131(15):154105. doi: 10.1063/1.3242273.
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Elementary steps in excited-state proton transfer.激发态质子转移的基本步骤。
J Phys Chem A. 2005 Jan 13;109(1):13-35. doi: 10.1021/jp047465m.
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Green's-function reaction dynamics: a particle-based approach for simulating biochemical networks in time and space.格林函数反应动力学:一种用于在时间和空间上模拟生化网络的基于粒子的方法。
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Introduction: 100 years of Brownian motion.引言:布朗运动的百年历程
Chaos. 2005 Jun;15(2):26101. doi: 10.1063/1.1895505.
6
Simulating biochemical networks at the particle level and in time and space: Green's function reaction dynamics.在粒子层面以及时间和空间维度上模拟生化网络:格林函数反应动力学
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