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铝土矿开采和氧化铝精炼的放射学评估。

Radiological assessment for bauxite mining and alumina refining.

作者信息

O'Connor Brian H, Donoghue A Michael, Manning Timothy J H, Chesson Barry J

机构信息

Centre for Materials Research, Department of Imaging and Applied Physics, Curtin University of Technology, GPO Box U1987, Perth, WA 6001, Australia.

出版信息

Ann Occup Hyg. 2013 Jan;57(1):63-76. doi: 10.1093/annhyg/mes052. Epub 2012 Sep 5.

Abstract

OBJECTIVE

Two international benchmarks assess whether the mining and processing of ores containing Naturally Occurring Radioactive Material (NORM) require management under radiological regulations set by local jurisdictions. First, the 1 Bq/g benchmark for radionuclide head of chain activity concentration determines whether materials may be excluded from radiological regulation. Second, processes may be exempted from radiological regulation where occupational above-background exposures for members of the workforce do not exceed 1 mSv/year. This is also the upper-limit of exposure prescribed for members of the public. Alcoa of Australia Limited (Alcoa) has undertaken radiological evaluations of the mining and processing of bauxite from the Darling Range of Western Australia since the 1980s. Short-term monitoring projects have demonstrated that above-background exposures for workers do not exceed 1 mSv/year. A whole-of-year evaluation of above-background, occupational radiological doses for bauxite mining, alumina refining and residue operations was conducted during 2008/2009 as part of the Alcoa NORM Quality Assurance System (NQAS). The NQAS has been guided by publications from the International Commission on Radiological Protection (ICRP), the International Atomic Energy Agency (IAEA) and the Australian Radiation Protection and Nuclear Safety Agency (ARPANSA). The NQAS has been developed specifically in response to implementation of the Australian National Directory on Radiation Protection (NDRP).

METHODS

Positional monitoring was undertaken to increase the accuracy of natural background levels required for correction of occupational exposures. This is important in view of the small increments in exposure that occur in bauxite mining, alumina refining and residue operations relative to natural background. Positional monitoring was also undertaken to assess the potential for exposure in operating locations. Personal monitoring was undertaken to characterise exposures in Similar Exposure Groups (SEGs). The monitoring was undertaken over 12 months, to provide annual average assessments of above-background doses, thereby reducing temporal variations, especially for radon exposures. The monitoring program concentrated on gamma and radon exposures, rather than gross alpha exposures, as past studies have shown that gross alpha exposures from inhalable dust for most of the workforce are small in comparison to combined gamma and radon exposures.

RESULTS

The natural background determinations were consistent with data in the literature for localities near Alcoa's mining, refining and residue operations in Western Australia, and also with UNSCEAR global data. Within the mining operations, there was further consistency between the above-background dose estimates and the local geochemistry, with slight elevation of dose levels in mining pits. Conservative estimates of above-background levels for the workforce have been made using an assumption of 100% occupancy (1920 hours per year) for the SEGs considered. Total incremental composite doses for individuals were clearly less than 1.0 mSv/year when gamma, radon progeny and gross alpha exposures were considered. This is despite the activity concentration of some materials being slightly higher than the benchmark of 1 Bq/g.

CONCLUSIONS

The results are consistent with previous monitoring and demonstrate compliance with the 1 mSv/year exemption level within mining, refining and residue operations. These results will be of value to bauxite mines and alumina refineries elsewhere in the world.

摘要

目的

两项国际基准评估含有天然放射性物质(NORM)的矿石开采和加工是否需要依据当地司法管辖区制定的放射法规进行管理。其一,链首放射性核素活度浓度的1贝可勒尔/克基准确定材料是否可免于放射法规监管。其二,若劳动力成员的职业背景以上照射不超过每年1毫希沃特,则相关工艺可免于放射法规监管。这也是规定的公众成员照射上限。自20世纪80年代以来,澳大利亚美铝有限公司(美铝)对西澳大利亚达令山脉的铝土矿开采和加工进行了放射学评估。短期监测项目表明,工人的背景以上照射不超过每年1毫希沃特。作为美铝NORM质量保证体系(NQAS)的一部分,在2008/2009年期间对铝土矿开采、氧化铝精炼和残渣作业的背景以上职业放射剂量进行了全年评估。NQAS以国际放射防护委员会(ICRP)、国际原子能机构(IAEA)和澳大利亚辐射防护与核安全局(ARPANSA)的出版物为指导。NQAS是专门针对澳大利亚国家辐射防护名录(NDRP)的实施而制定的。

方法

进行位置监测以提高校正职业照射所需的自然本底水平的准确性。鉴于铝土矿开采、氧化铝精炼和残渣作业中相对于自然本底而言照射的增量较小,这一点很重要。还进行位置监测以评估作业地点的照射可能性。进行个人监测以确定类似照射组(SEG)中的照射情况。监测为期12个月,以提供背景以上剂量的年度平均评估,从而减少时间变化,特别是对于氡照射。监测计划集中于伽马和氡照射,而非总阿尔法照射,因为过去的研究表明,与伽马和氡的综合照射相比,大多数劳动力吸入粉尘中的总阿尔法照射量较小。

结果

自然本底测定结果与美铝在西澳大利亚的采矿、精炼和残渣作业附近地区的文献数据一致,也与联合国原子辐射效应科学委员会(UNSCEAR)的全球数据一致。在采矿作业中,背景以上剂量估计值与当地地球化学之间进一步保持一致,矿坑中的剂量水平略有升高。对于所考虑的SEG,使用100%占用率(每年1920小时)的假设对劳动力的背景以上水平进行了保守估计。当考虑伽马、氡子体和总阿尔法照射时,个体的总增量复合剂量明显低于每年1.0毫希沃特。尽管某些材料的活度浓度略高于1贝可勒尔/克的基准。

结论

结果与先前的监测一致,并表明在采矿、精炼和残渣作业中符合每年1毫希沃特的豁免水平。这些结果将对世界其他地方的铝土矿和氧化铝精炼厂具有价值。

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