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[评估光核活化用于退役医用直线加速器的清除]

[Evaluating photonuclear activation for clearance of decommissioned medical linear accelerators].

作者信息

Shida Koichi, Isobe Tomonori, Takada Kenta, Kobayashi Daisuke, Tadano Kiichi, Takahashi Hideki, Seki Masashi, Yokota Hiroshi, Sakurai Hideyuki, Sakae Takeji

机构信息

Graduate School of Comprehensive Human Sciences, University of Tsukuba, Japan.

出版信息

Igaku Butsuri. 2011;31(2):33-9.

Abstract

In a linear accelerator (linac) that operates at greater than an accelerating energy of 10 MV, neutrons are generated by a photonuclear reaction and the head section of the linac becomes radioactive. The purpose of this research is to obtain data for ensuring the safety of linac decommissioning and upgrading. The decommissioned linac investigated in this study was a Clinac 2100 C/D (Varian) installed in April 1999. Its total time of use was 2757.7 h (equivalent to 496,386 Gy). The dosage for its last three months of use was 7213.67 Gy. After being allowed to sit for a 7-day cooling period, the apparatus was disassembled and the parts of the gantry head portion were removed. The ambient dose equivalent rates, H*(10), (microSv/h) from the removed parts were measured in air, at a location with low background, by using a gamma ray scintillation survey meter. The target was also analyzed with an HP-Ge semiconductor detector, in order to identify the nuclides responsible for the observed radiation. On day 7 after the last use of the linac, the ambient dose equivalent rates, H*(10), (microSv/h) in air at the surface of all parts, except the target and the beryllium window, were within the limit of normal background radiation. The measured value (microSv/h) for the beryllium window decreased to within the background limit on day 10. The measured value (microSv/h) of the target decreased to about 1.5 times the background on day 19. At a distance of 10 cm, all the parts were within the background limit after the initial 7-day cooling period. In the analysis of the target with the HP-Ge semiconductor detector, peaks at 125, 333, 352, 356, 426, 511, 583, 609, 689, 811, 835, 911, 969, 1091, 1099, 1120, 1173, 1238, 1292, 1333, 1461 and 1764keV were detected on day 23. Seven months after the linac was last used, peaks were detected at 352, 511, 583, 609, 835, 911, 969, 1120, 1173, 1238, 1333, 1461 and 1764 keV. From these results, the natural radioactive nuclides can be assigned as 40K, 208Tl, 214Pb, 214Bi and 228Ac; the short half-life nuclides can be assigned as 59Fe, 58Co, 185W and 196Au; and the long half-life nuclides can be assigned as 54Mn and 60Co. These results show that photonuclear activation of parts is important in regard to clearance. Currently, there are no regulations that specify criteria for evaluating radioactivation. Such criteria are needed to establish suitable protocols for the clearance of radioactivated materials.

摘要

在加速能量大于10 MV运行的直线加速器(linac)中,光核反应会产生中子,直线加速器的头部会变得具有放射性。本研究的目的是获取数据,以确保直线加速器退役和升级的安全性。本研究中调查的退役直线加速器是1999年4月安装的Clinac 2100 C/D(瓦里安公司)。其总使用时间为2757.7小时(相当于496,386戈瑞)。其最后三个月的使用剂量为7213.67戈瑞。在静置7天冷却期后,该设备被拆卸,机架头部部分的部件被移除。使用伽马射线闪烁测量仪在低本底的空气中测量移除部件的环境剂量当量率H*(10)(微希沃特/小时)。还使用HP-Ge半导体探测器对靶进行分析,以识别造成观测到的辐射的核素。直线加速器最后一次使用后的第7天,除靶和铍窗外,所有部件表面空气中的环境剂量当量率H*(10)(微希沃特/小时)均在正常本底辐射限值内。铍窗的测量值(微希沃特/小时)在第10天降至本底限值内。靶的测量值(微希沃特/小时)在第19天降至约为本底的1.5倍。在10厘米的距离处,经过最初7天的冷却期后,所有部件均在本底限值内。在使用HP-Ge半导体探测器对靶进行的分析中,在第23天检测到125、333、352、356、426、511、583、609、689、811、835、911、969、1091、1099、1120、1173、1238、1292、1333、1461和1764keV处的峰。直线加速器最后一次使用七个月后,在352、511、583、609、835、911、969、1120、1173、1238、1333、1461和1764keV处检测到峰。根据这些结果,天然放射性核素可确定为40K、208Tl、214Pb、214Bi和228Ac;短半衰期核素可确定为59Fe、58Co、185W和196Au;长半衰期核素可确定为54Mn和60Co。这些结果表明,部件的光核活化对于清理而言很重要。目前,尚无规定明确评估放射性活化的标准。需要这样的标准来制定清理放射性活化材料的合适方案。

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