Quantum Phase Electronics Center and Department of Applied Physics, University of Tokyo, Tokyo 113-8656, Japan.
Phys Rev Lett. 2012 Jun 22;108(25):257401. doi: 10.1103/PhysRevLett.108.257401. Epub 2012 Jun 19.
We have investigated the ultrafast spin dynamics in EuO thin films by time-resolved Faraday rotation spectroscopy. The photoinduced magnetization is found to be increased in a transient manner, accompanied with subsequent demagnetization. The dynamical magnetization enhancement showed a maximum slightly below the Curie temperature with prolonged tails toward both lower and higher temperatures and dominates the demagnetization counterpart at 55 K. The magnetization enhancement component decays in ~1 ns. The realization of the transient collective ordering is attributable to the enhancement of the f-d exchange interaction.
我们通过时间分辨法拉第旋转光谱研究了 EuO 薄膜中的超快自旋动力学。发现光致磁化在瞬态方式下增加,伴随着随后的退磁。动态磁化增强在居里温度以下略呈最大值,并向低温和高温两侧延长尾巴,在 55 K 时主导退磁对应部分。磁化增强分量在~1 ns 内衰减。瞬态集体有序的实现归因于 f-d 交换相互作用的增强。