Department of Physics, Oregon State University, Corvallis, Oregon 97331, USA.
Phys Rev Lett. 2012 Jun 29;108(26):267402. doi: 10.1103/PhysRevLett.108.267402. Epub 2012 Jun 26.
Interactions of few-cycle terahertz pulses with the induced optical polarization in a quantum-well microcavity reveal that the lower and higher exciton-polariton modes together with the optically forbidden 2p-exciton state form a unique Λ-type three-level system. Pronounced nonlinearities are observed via time-resolved strong-terahertz and weak-optical excitation spectroscopy and explained with a fully microscopic theory. The results show that the terahertz pulses strongly couple the exciton-polariton states to the 2p-exciton state while no resonant transition between the two polariton levels is observed.
在量子阱微腔中,与感应光学极化相互作用的少周期太赫兹脉冲揭示了低能和高能激子极化激元模式以及光学禁戒的 2p-激子态共同构成了独特的 Λ 型三能级系统。通过时间分辨强太赫兹和弱光学激发光谱学观察到明显的非线性,并通过全微观理论进行了解释。结果表明,太赫兹脉冲强烈地将激子极化激元态与 2p-激子态耦合,而在两个极化激元能级之间没有观察到共振跃迁。