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揭示亮激子极化激元凝聚体的黑暗面。

Revealing the dark side of a bright exciton-polariton condensate.

机构信息

Department of Physics, University of Regensburg, 93040 Regensburg, Germany.

CNRS-Laboratoire de Photonique et Nanostructures, Route de Nozay, 91460 Marcoussis, France.

出版信息

Nat Commun. 2014 Aug 13;5:4648. doi: 10.1038/ncomms5648.

Abstract

Condensation of bosons causes spectacular phenomena such as superfluidity or superconductivity. Understanding the nature of the condensed particles is crucial for active control of such quantum phases. Fascinating possibilities emerge from condensates of light-matter-coupled excitations, such as exciton-polaritons, photons hybridized with hydrogen-like bound electron-hole pairs. So far, only the photon component has been resolved, while even the mere existence of excitons in the condensed regime has been challenged. Here we trace the matter component of polariton condensates by monitoring intra-excitonic terahertz transitions. We study how a reservoir of optically dark excitons forms and feeds the degenerate state. Unlike atomic gases, the atom-like transition in excitons is dramatically renormalized on macroscopic ground state population. Our results establish fundamental differences between polariton condensation and photon lasing and open possibilities for coherent control of condensates.

摘要

玻色子凝聚会导致超流或超导等壮观现象。理解凝聚粒子的性质对于主动控制这种量子相至关重要。光物质耦合激发的凝聚体,如激子极化激元、与类氢束缚电子空穴对混合的光子,带来了令人着迷的可能性。到目前为止,人们只解析了光子成分,而凝聚态中激子的存在本身就受到了挑战。在这里,我们通过监测太赫兹范围内的内激子跃迁来追踪极化激元凝聚体的物质成分。我们研究了光学暗激子库如何形成并为简并态提供物质。与原子气体不同,激子中的类原子跃迁在宏观基态下会被剧烈重整化。我们的结果揭示了极化激元凝聚与光子激射之间的根本差异,并为凝聚体的相干控制开辟了可能性。

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