2H-四苯基卟啉在Cu(111)上进行自金属化反应的活化能。 - Suppr

Activation energy for the self-metalation reaction of 2H-tetraphenylporphyrin on Cu(111).

作者信息

Ditze Stefanie, Stark Michael, Drost Martin, Buchner Florian, Steinrück Hans-Peter, Marbach Hubertus

机构信息

Lehrstuhl für Physikalische Chemie II and Interdisciplinary Center for Molecular Materials, Universität Erlangen-Nürnberg, Egerlandstrasse 3, 91058 Erlangen, Germany.

出版信息

Angew Chem Int Ed Engl. 2012 Oct 22;51(43):10898-901. doi: 10.1002/anie.201205464. Epub 2012 Sep 26.

DOI:10.1002/anie.201205464

PMID:23012215

Abstract

摘要

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Activation energy for the self-metalation reaction of 2H-tetraphenylporphyrin on Cu(111).

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Activation energy for the self-metalation reaction of 2H-tetraphenylporphyrin on Cu(111).

Angew Chem Int Ed Engl. 2012 Oct 22;51(43):10898-901. doi: 10.1002/anie.201205464. Epub 2012 Sep 26.

Coverage- and temperature-dependent metalation and dehydrogenation of tetraphenylporphyrin on Cu(111).

Chemistry. 2014 Jul 14;20(29):8948-53. doi: 10.1002/chem.201402420. Epub 2014 Jun 25.

Self-metalation of 2H-tetraphenylporphyrin on Cu(111): an x-ray spectroscopy study.

J Chem Phys. 2012 Jan 7;136(1):014705. doi: 10.1063/1.3674165.

Principle and mechanism of direct porphyrin metalation: joint experimental and theoretical investigation.

J Am Chem Soc. 2007 Aug 1;129(30):9476-83. doi: 10.1021/ja072360t. Epub 2007 Jul 11.

Evidence for the formation of an intermediate complex in the direct metalation of tetra(4-bromophenyl)-porphyrin on the Cu(111) surface.

Chem Commun (Camb). 2011 Nov 28;47(44):12134-6. doi: 10.1039/c1cc15241f. Epub 2011 Oct 13.

Dynamics of molecular self-ordering in tetraphenyl porphyrin monolayers on metallic substrates.

Nanotechnology. 2009 Jul 8;20(27):275602. doi: 10.1088/0957-4484/20/27/275602. Epub 2009 Jun 17.

Thermally and vibrationally induced tautomerization of single porphycene molecules on a Cu(110) surface.

Phys Rev Lett. 2013 Dec 13;111(24):246101. doi: 10.1103/PhysRevLett.111.246101. Epub 2013 Dec 11.

A small molecule walks along a surface between porphyrin fences that are assembled in situ.

Angew Chem Int Ed Engl. 2015 Jun 8;54(24):7101-5. doi: 10.1002/anie.201502153. Epub 2015 Apr 29.

Electrochemical reactions at a porphyrin-copper interface.

Phys Chem Chem Phys. 2009 Jul 14;11(26):5422-30. doi: 10.1039/b807075j. Epub 2009 Apr 23.

Self-assembly of flexible one-dimensional coordination polymers on metal surfaces.

J Am Chem Soc. 2010 May 19;132(19):6783-90. doi: 10.1021/ja1010527.

引用本文的文献

On-Surface Synthesis of Na-Porphyrins Using NaCl as a Convenient Na Source.

Precis Chem. 2023 Apr 5;1(4):226-232. doi: 10.1021/prechem.3c00014. eCollection 2023 Jun 26.

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Chemistry. 2025 Jul 17;31(40):e202500998. doi: 10.1002/chem.202500998. Epub 2025 Jul 1.

Thermally Activated on-Surface Self-Metalation of Pd-Phthalocyanines.

Chemistry. 2025 May 19;31(28):e202500944. doi: 10.1002/chem.202500944. Epub 2025 Apr 18.

Formation of Highly Ordered Molecular Porous 2D Networks from Cyano-Functionalized Porphyrins on Cu(111).

Chemistry. 2020 Oct 21;26(59):13408-13418. doi: 10.1002/chem.202001980. Epub 2020 Sep 17.

Self-Metalation of Anchored Porphyrins on Atomically Defined Cobalt Oxide Surfaces: In situ Studies by Surface Vibrational Spectroscopy.

Chemistry. 2020 Sep 25;26(54):12445-12453. doi: 10.1002/chem.202001331. Epub 2020 Sep 3.

Conformation Controls Mobility: 2H-Tetranaphthylporphyrins on Cu(111).

Chemphyschem. 2020 Mar 4;21(5):423-427. doi: 10.1002/cphc.201901135. Epub 2020 Feb 17.

Metalation of tetraphenylporphyrin with nickel on a TiO2(110)-1 × 2 surface.

Nanoscale. 2016 Jan 14;8(2):1123-1132. doi: 10.1039/c5nr03134f.

Porphyrins at interfaces.

Nat Chem. 2015 Feb;7(2):105-20. doi: 10.1038/nchem.2159.

Activation energy for the self-metalation reaction of 2H-tetraphenylporphyrin on Cu(111).

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