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福岛第一核电站以南 70 公里的茨城县沿海地区放射性铯的沉降和再悬浮。

Sedimentation and remobilization of radiocesium in the coastal area of Ibaraki, 70 km south of the Fukushima Dai-ichi Nuclear Power Plant.

机构信息

Research Group for Environmental Science, Japan Atomic Energy Agency, Tokai-mura, Ibaraki, Japan.

出版信息

Environ Monit Assess. 2013 Jul;185(7):5419-33. doi: 10.1007/s10661-012-2956-7. Epub 2012 Nov 13.

Abstract

Sedimentation and remobilization processes of radiocesium were investigated from time-series observations at nine stations in the coastal area of Ibaraki, 70-110 km south of the Fukushima Dai-ichi Nuclear Power Plant (1FNPP). Sediment samples were collected four times between June 2011 and January 2012, and concentrations of radiocesium as well as sediment properties such as grain size and elemental compositions were analyzed. Cumulative inventory of (137)Cs in sediment (0-10 cm) ranged between 4 × 10(3) and 3 × 10(4) Bq/m(2) as of January 2012. This amount was generally higher at stations nearer 1FNPP and has remained at the same level since August 2011. From these results, it can be inferred that dissolved radiocesium advected southward from the region adjacent to the 1FNPP and was deposited to the sediment of the study area in the early stage after the accident. The incorporation of radiocesium into sediments was almost irreversible, and higher concentrations of (137)Cs were obtained from the finer-grained fraction of sediments. In the northern offshore stations, resuspension of the fine-grained sediments formed a high-turbidity layer 10-20 m above the seabed. These results indicate that radiocesium-enriched fine particles were transported from the coast to offshore regions through the bottom high-turbidity layer.

摘要

从福岛第一核电站(1FNPP)以南 70-110 公里的茨城县沿海地区九个站位的时间序列观测中,研究了放射性铯的沉降和再悬浮过程。2011 年 6 月至 2012 年 1 月期间,共采集了四次沉积物样品,并分析了放射性铯浓度以及沉积物特性,如粒度和元素组成。截至 2012 年 1 月,沉积物(0-10cm)中(137)Cs 的累积库存为 4×10(3)至 3×10(4)Bq/m(2)。这一数量在靠近 1FNPP 的站位通常较高,并自 2011 年 8 月以来一直保持在同一水平。从这些结果可以推断,从 1FNPP 附近区域沿水流向南输送的溶解态放射性铯在事故发生后不久就被沉积到研究区域的沉积物中。放射性铯进入沉积物的过程几乎是不可逆的,并且从沉积物的较细颗粒部分获得了更高浓度的(137)Cs。在北部近岸站位,细颗粒沉积物的再悬浮形成了一个海底上方 10-20 米高的高浊度层。这些结果表明,富含放射性铯的细颗粒通过底部高浊度层从海岸输送到近海区域。

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