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非厄米等离子体超材料中的量子 Hanle 效应及偏振转换的模拟。

Analogue of the quantum Hanle effect and polarization conversion in non-Hermitian plasmonic metamaterials.

机构信息

Department of Physics, King's College London, Strand, London WC2R 2LS, United Kingdom.

出版信息

Nano Lett. 2012 Dec 12;12(12):6309-14. doi: 10.1021/nl3034174. Epub 2012 Nov 21.

Abstract

The Hanle effect, one of the first manifestations of quantum theory introducing the concept of coherent superposition between pure states, plays a key role in numerous aspects of science varying from applicative spectroscopy to fundamental astrophysical investigations. Optical analogues of quantum effects help to achieve deeper understanding of quantum phenomena and, in turn, to develop cross-disciplinary approaches to realizations of new applications in photonics. Here we show that metallic nanostructures can be designed to exhibit a plasmonic analogue of the quantum Hanle effect and the associated polarization rotation. In the original Hanle effect, time-reversal symmetry is broken by a static magnetic field. We achieve this by introducing dissipative level crossing of localized surface plasmons due to nonuniform losses, designed using a non-Hermitian formulation of quantum mechanics. Such artificial plasmonic "atoms" have been shown to exhibit strong circular birefringence and circular dichroism which depends on the value of loss or gain in the metal-dielectric nanostructure.

摘要

Hanle 效应是量子理论首次引入纯态相干叠加概念的表现之一,在从应用光谱学到基础天体物理研究等众多科学领域都起着关键作用。量子效应的光学类似物有助于更深入地理解量子现象,并反过来为在光子学中实现新应用的跨学科方法提供了途径。在这里,我们展示了可以设计金属纳米结构以表现出量子 Hanle 效应及相关偏振旋转的等离子体类似物。在原始的 Hanle 效应中,时间反演对称性被静态磁场打破。我们通过引入由于非均匀损耗而导致的局域表面等离激元的耗散能级交叉来实现这一点,这是使用量子力学的非厄米形式来设计的。已经表明,这种人工等离子体“原子”表现出强烈的圆双折射和圆二色性,其取决于金属-电介质纳米结构中的损耗或增益值。

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