Duval M, Arnold L J
Centro Nacional de Investigación sobre la Evolución Humana, CENIEH, Paseo Sierra de Atapuerca s/n, Burgos, Spain.
Appl Radiat Isot. 2013 Apr;74:36-45. doi: 10.1016/j.apradiso.2012.12.006. Epub 2012 Dec 20.
Results are presented for a series of replicate in situ gamma spectrometry measurements (n=20) made in natural sedimentary contexts using LaBr3(Ce) and NaI(Tl) probes. For both types of detectors, gamma dose rates were calculated using the "threshold" technique (Murray et al., 1978), and compared with results obtained previously by Arnold et al. (2012) using the "windows" technique (Aitken, 1985). Our results show that gamma dose rates obtained using these two techniques are consistent at 1σ for a given probe, and that the threshold technique yields reproducible results for the LaBr3(Ce) and NaI(Tl) probes. In comparison with the energy windows approach, the threshold approach offers an improvement in the precision with which gamma dose rates can be determined using the LaBr3(Ce) probe. The potential of an alternative threshold approach (the "energy threshold" approach of Guérin and Mercier, 2011) was also tested for both probe types, and the resultant gamma dose rates were found to be in agreement with those obtained using the standard threshold and energy windows techniques. Our results provide new insights into methods and instrumentation used for assessing in situ gamma dose rates in Electron Spin Resonance (ESR) and Luminescence dating. We conclude that LaBr3(Ce) probes can reliably be used for portable gamma dosimetry in low level activity sedimentary environments (500-1500μGy/a) when using the threshold approach, provided that their non-negligible internal background activities (equivalent to ∼758μGy/a for our probe) are accurately assessed and subtracted from gamma ray spectra measured in the field. Our results also suggest that there may be some minor merit in applying an internal background-subtraction procedure to NaI(Tl) gamma ray spectra when using the threshold technique, in spite of the lower intrinsic activities of NaI(Tl) detectors.
本文展示了一系列在天然沉积环境中使用溴化镧(铈)和碘化钠(铊)探测器进行的原位伽马能谱重复测量结果(n = 20)。对于这两种探测器,伽马剂量率均采用“阈值”技术(Murray等人,1978年)进行计算,并与Arnold等人(2012年)使用“窗口”技术(Aitken,1985年)先前获得的结果进行比较。我们的结果表明,对于给定的探测器,使用这两种技术获得的伽马剂量率在1σ水平上是一致的,并且阈值技术对溴化镧(铈)和碘化钠(铊)探测器产生了可重复的结果。与能量窗口方法相比,阈值方法在使用溴化镧(铈)探测器确定伽马剂量率的精度方面有所提高。还对两种探测器类型测试了另一种阈值方法(Guérin和Mercier,2011年的“能量阈值”方法)的潜力,发现所得伽马剂量率与使用标准阈值和能量窗口技术获得的结果一致。我们的结果为电子自旋共振(ESR)和发光测年中用于评估原位伽马剂量率的方法和仪器提供了新的见解。我们得出结论,当使用阈值方法时,溴化镧(铈)探测器能够可靠地用于低水平放射性沉积环境(500 - 1500μGy/a)中的便携式伽马剂量测定,前提是其不可忽略的内部本底放射性(对于我们的探测器相当于约758μGy/a)得到准确评估并从现场测量的伽马射线光谱中扣除。我们的结果还表明,尽管碘化钠(铊)探测器的固有放射性较低,但在使用阈值技术时,对碘化钠(铊)伽马射线光谱应用内部本底扣除程序可能有一些微小的优势。